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@article{1163807,
author = {Lohmann, Rainer and Klánová, Jana and Kukučka, Petr and Yonis, Shifra and Bollinger, Kevyn},
article_location = {WASHINGTON},
article_number = {24},
doi = {http://dx.doi.org/10.1021/es403494b},
keywords = {POLYBROMINATED DIPHENYL ETHERS; PERSISTENT ORGANIC POLLUTANTS; POLYCHLORINATED-BIPHENYLS; PHYSICOCHEMICAL PROPERTIES; PERFLUORINATED ACIDS; ENVIRONMENTAL FATE; SURFACE SEAWATER; DRY DEPOSITION; AIR-WATER; PCBS},
language = {eng},
issn = {0013-936X},
journal = {ENVIRONMENTAL SCIENCE andTECHNOLOGY},
title = {Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean},
volume = {47},
year = {2013}
}
TY - JOUR
ID - 1163807
AU - Lohmann, Rainer - Klánová, Jana - Kukučka, Petr - Yonis, Shifra - Bollinger, Kevyn
PY - 2013
TI - Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean
JF - ENVIRONMENTAL SCIENCE andTECHNOLOGY
VL - 47
IS - 24
SP - 13967-13975
EP - 13967-13975
PB - AMER CHEMICAL SOC
SN - 0013936X
KW - POLYBROMINATED DIPHENYL ETHERS
KW - PERSISTENT ORGANIC POLLUTANTS
KW - POLYCHLORINATED-BIPHENYLS
KW - PHYSICOCHEMICAL PROPERTIES
KW - PERFLUORINATED ACIDS
KW - ENVIRONMENTAL FATE
KW - SURFACE SEAWATER
KW - DRY DEPOSITION
KW - AIR-WATER
KW - PCBS
N2 - Little is known about the fate of polybrominated diphenylethers (PBDEs) across the Oceans. Air and water were sampled using both active and passive polyethylene samplers on an east-west transect across the tropical Atlantic Ocean in 2009 and analyzed for PBDEs. Typical particle-bound concentrations of PBDEs in the surface water were low, at <1 pg L-1. Truly dissolved concentrations from passive samplers were similar to 40.5 pg L-1 for BDE 47 and around 0.1 pg L-1 for BDEs 28, 99, and 100 (results from active samples were compromised). In the atmosphere, particle-bound BDE 209 dominated overall concentrations (median 1.2 pg m(-3)), followed by BDE 99 (0.13 pg m(-3)). Gas-phase concentrations based on passive samplers were 1-8 pg m(-3) for BDE 47 and <= 4 pg m(-3) for BDE 99. Net air-water exchange gradients strongly favored gas-phase deposition of PBDEs into the water. Net gas-phase deposition fluxes ranged from tens of pg m(-2) day(-1) for BDEs 28 and 85 to around 1 ng m(-2) day(-1) for BDE 47, 99, and 209. Settling fluxes of particle-bound PBDEs in the atmosphere and surface water were around 50 pg m(-2) day(-1) for BDE 47 and <10 pg m(-2) day(-1) for the other congeners.
ER -
LOHMANN, Rainer, Jana KLÁNOVÁ, Petr KUKUČKA, Shifra YONIS and Kevyn BOLLINGER. Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean. \textit{ENVIRONMENTAL SCIENCE andTECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2013, vol.~47, No~24, p.~13967-13975. ISSN~0013-936X. Available from: https://dx.doi.org/10.1021/es403494b.
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