Long-range atmospheric transport of PAHs, PCBs and PBDEs to the
central and eastern Mediterranean and changes of PCB and PBDE
congener patterns in summer 2010

J 2015

Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010

MULDER, Marie Daniëlle, Angelika HEIL, Petr KUKUČKA, Jan KUTA, Petra PŘIBYLOVÁ et. al.

Basic information

Original name

Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010

Authors

MULDER, Marie Daniëlle (528 Netherlands, belonging to the institution), Angelika HEIL (276 Germany), Petr KUKUČKA (203 Czech Republic, belonging to the institution), Jan KUTA (203 Czech Republic, belonging to the institution), Petra PŘIBYLOVÁ (203 Czech Republic, belonging to the institution), Roman PROKEŠ (203 Czech Republic, belonging to the institution) and Gerhard LAMMEL (276 Germany, guarantor, belonging to the institution)

Edition

Atmospheric Environment, OXFORD (ENGLAND), Pergamon Press, 2015, 1352-2310

Other information

Language

English

Type of outcome

Článek v odborném periodiku

Field of Study

10511 Environmental sciences

Country of publisher

United Kingdom of Great Britain and Northern Ireland

Confidentiality degree

není předmětem státního či obchodního tajemství

References:

URL

Impact factor

Impact factor: 3.459

RIV identification code

RIV/00216224:14310/15:00081585

Organization unit

Faculty of Science

DOI

http://dx.doi.org/10.1016/j.atmosenv.2015.03.044

UT WoS

000355026100006

Keywords in English

Long-range transport; Marine environment; Persistent organic pollutants; Mediterranean

Abstract

V originále

The central and eastern Mediterranean is a receptor area for persistent organic pollutants (POPs) emitted in western, central and eastern Europe, particularly during summer. Atmospheric concentrations of PCBs, DDXs, PBDEs, penta- and hexachlorobenzene were measured during a ship-borne survey in the summer of 2010. The concentration of PCBs (sum of 7 congeners) was 3.61 (2.08-7.72) pg m(-3), of which 6.7% was associated with the particulate phase. The mean concentration of DDT isoi-ners and their metabolites, DDE and DDD, was 2.60 (0.46-7.60) pg m(-3) (particulate mass fraction theta = 0.097), of penta- and hexachlorobenzene 0.22 (<039-2.80) pg m(-3) and 6.29 (2.48-24.16) pg m(-3), respectively, and of PBDEs (sum of 8 congeners) 7.31 (2.80-19.89) pg m(-3). The air masses studied had been transported mostly across central Europe, some crossing western Europe. The observed changes of PCB congener patterns along transport routes are in agreement with the perception that the reaction with the OH radical is dominating PCB atmospheric lifetime, and indicate an overestimation of the second order gas-phase reaction rate coefficient of PCB:153 with OH by structure-activity relationship.

Links

ED0001/01/01, research and development project

Name: CETOCOEN

GAP503/11/1230, research and development project

Name: Perzistentní organické polutanty v atmosférických aerosolech: Procesy, které ovlivňují dálkový transport v Evropě.

Investor: Czech Science Foundation

LM2011028, research and development project

Name: RECETOX ? Národní infrastruktura pro výzkum toxických látek v prostředí

Investor: Ministry of Education, Youth and Sports of the CR

LO1214, research and development project

Name: Centrum pro výzkum toxických látek v prostředí (Acronym: RECETOX)

Investor: Ministry of Education, Youth and Sports of the CR

Citovat

MULDER, Marie Daniëlle, Angelika HEIL, Petr KUKUČKA, Jan KUTA, Petra PŘIBYLOVÁ, Roman PROKEŠ and Gerhard LAMMEL. Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010. Atmospheric Environment. OXFORD (ENGLAND): Pergamon Press, 2015, vol. 111, JUNE, p. 51-59. ISSN 1352-2310. Available from: https://dx.doi.org/10.1016/j.atmosenv.2015.03.044.

@article{1336052,
   author = {Mulder, Marie Daniëlle and Heil, Angelika and Kukučka, Petr and Kuta, Jan and Přibylová, Petra and Prokeš, Roman and Lammel, Gerhard},
   article_location = {OXFORD (ENGLAND)},
   article_number = {JUNE},
   doi = {http://dx.doi.org/10.1016/j.atmosenv.2015.03.044},
   keywords = {Long-range transport; Marine environment; Persistent organic pollutants; Mediterranean},
   language = {eng},
   issn = {1352-2310},
   journal = {Atmospheric Environment},
   title = {Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010},
   url = {http://www.sciencedirect.com/science/article/pii/S135223101500268X},
   volume = {111},
   year = {2015}
}

TY  - JOUR
ID  - 1336052
AU  - Mulder, Marie Daniëlle - Heil, Angelika - Kukučka, Petr - Kuta, Jan - Přibylová, Petra - Prokeš, Roman - Lammel, Gerhard
PY  - 2015
TI  - Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010
JF  - Atmospheric Environment
VL  - 111
IS  - JUNE
SP  - 51-59
EP  - 51-59
PB  - Pergamon Press
SN  - 13522310
KW  - Long-range transport
KW  - Marine environment
KW  - Persistent organic pollutants
KW  - Mediterranean
UR  - http://www.sciencedirect.com/science/article/pii/S135223101500268X
L2  - http://www.sciencedirect.com/science/article/pii/S135223101500268X
N2  - The central and eastern Mediterranean is a receptor area for persistent organic pollutants (POPs) emitted in western, central and eastern Europe, particularly during summer. Atmospheric concentrations of PCBs, DDXs, PBDEs, penta- and hexachlorobenzene were measured during a ship-borne survey in the summer of 2010. The concentration of PCBs (sum of 7 congeners) was 3.61 (2.08-7.72) pg m(-3), of which 6.7% was associated with the particulate phase. The mean concentration of DDT isoi-ners and their metabolites, DDE and DDD, was 2.60 (0.46-7.60) pg m(-3) (particulate mass fraction theta = 0.097), of penta- and hexachlorobenzene 0.22 (<039-2.80) pg m(-3) and 6.29 (2.48-24.16) pg m(-3), respectively, and of PBDEs (sum of 8 congeners) 7.31 (2.80-19.89) pg m(-3). The air masses studied had been transported mostly across central Europe, some crossing western Europe. The observed changes of PCB congener patterns along transport routes are in agreement with the perception that the reaction with the OH radical is dominating PCB atmospheric lifetime, and indicate an overestimation of the second order gas-phase reaction rate coefficient of PCB:153 with OH by structure-activity relationship.
ER  -

MULDER, Marie Dani$\backslash$''elle, Angelika HEIL, Petr KUKUČKA, Jan KUTA, Petra PŘIBYLOVÁ, Roman PROKEŠ and Gerhard LAMMEL. Long-range atmospheric transport of PAHs, PCBs and PBDEs to the central and eastern Mediterranean and changes of PCB and PBDE congener patterns in summer 2010. \textit{Atmospheric Environment}. OXFORD (ENGLAND): Pergamon Press, 2015, vol.~111, JUNE, p.~51-59. ISSN~1352-2310. Available from: https://dx.doi.org/10.1016/j.atmosenv.2015.03.044.

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