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@article{1371893, author = {Degrendele, Celine and Audy, Ondřej and Hofman, Jakub and Kucerik, Jiří and Kukučka, Petr and Mulder, Marie Daniëlle and Přibylová, Petra and Prokeš, Roman and Sáňka, Milan and Schaumann, Gabriele E. and Lammel, Gerhard}, article_location = {WASHINGTON}, article_number = {8}, doi = {http://dx.doi.org/10.1021/acs.est.5b05671}, keywords = {POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; CENTRAL TIBETAN PLATEAU; ORGANOCHLORINE PESTICIDES; POLYCHLORINATED-BIPHENYLS; PARTITION-COEFFICIENTS; SURFACE SOIL; BLACK CARBON; SPATIAL-DISTRIBUTION; ATMOSPHERIC CONCENTRATIONS}, language = {eng}, issn = {0013-936X}, journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY}, title = {Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area}, url = {http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671}, volume = {50}, year = {2016} }
TY - JOUR ID - 1371893 AU - Degrendele, Celine - Audy, Ondřej - Hofman, Jakub - Kucerik, Jiří - Kukučka, Petr - Mulder, Marie Daniëlle - Přibylová, Petra - Prokeš, Roman - Sáňka, Milan - Schaumann, Gabriele E. - Lammel, Gerhard PY - 2016 TI - Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area JF - ENVIRONMENTAL SCIENCE & TECHNOLOGY VL - 50 IS - 8 SP - 4278-4288 EP - 4278-4288 PB - AMER CHEMICAL SOC SN - 0013936X KW - POLYCYCLIC AROMATIC-HYDROCARBONS KW - POLYBROMINATED DIPHENYL ETHERS KW - CENTRAL TIBETAN PLATEAU KW - ORGANOCHLORINE PESTICIDES KW - POLYCHLORINATED-BIPHENYLS KW - PARTITION-COEFFICIENTS KW - SURFACE SOIL KW - BLACK CARBON KW - SPATIAL-DISTRIBUTION KW - ATMOSPHERIC CONCENTRATIONS UR - http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671 L2 - http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671 N2 - Concentrations of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), organochlorine pesticides (OCPs), and polybrominated diphenyl ethers (PBDEs) in air and soil, their fugacities, and the experimental soil-air partitioning coefficient (K-SA) were determined at two background sites in the Gt. Hungarian Plain in August 2013. The concentrations of the semivolatile organic compounds (SOCs) in the soil were not correlated with the organic carbon content but with two indirect parameters of mineralization and aromaticity, suggesting that soil organic matter quality is an important parameter affecting the sorption of SOCs onto soils. Predictions based on the assumption that absorption is the dominant process were in good agreement with the measurements for PAHs, OCPs, and the low chlorinated PCBs. In general, soils were found to be a source of PAHs, high chlorinated PCBs, the majority of OCPs and PBDEs, and a sink for the low chlorinated PCBs and gamma-hexachlorocyclohexane. Diurnal variations in the direction of the soil-air exchange were found for two compounds (i.e., pentachlorobenzene and p,p'-dichlorodiphenyldichloroethane), with volatilization during the day and deposition in the night. The concentrations of most SOCs in the near-ground atmosphere were dominated by revolatilization from the soil. ER -
DEGRENDELE, Celine, Ondřej AUDY, Jakub HOFMAN, Jiří KUCERIK, Petr KUKUČKA, Marie Dani$\backslash$''elle MULDER, Petra PŘIBYLOVÁ, Roman PROKEŠ, Milan SÁŇKA, Gabriele E. SCHAUMANN and Gerhard LAMMEL. Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2016, vol.~50, No~8, p.~4278-4288. ISSN~0013-936X. Available from: https://dx.doi.org/10.1021/acs.est.5b05671.
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