| DVOŘÁK, Pavel, Marek TALÁBA, Adam OBRUSNÍK, Kratzer JAN and Dědina JIŘÍ. Concentration of atomic hydrogen in a dielectric barrier discharge measured by two-photon absorption fluorescence. Plasma Sources Science and Technology. Bristol: IOP PUBLISHING LTD, 2017, vol. 26, No 8, p. nestránkováno, 13 pp. ISSN 0963-0252. Available from: https://dx.doi.org/10.1088/1361-6595/aa76f7. |
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@article{1385997,
author = {Dvořák, Pavel and Talába, Marek and Obrusník, Adam and Jan, Kratzer and Jiří, Dědina},
article_location = {Bristol},
article_number = {8},
doi = {http://dx.doi.org/10.1088/1361-6595/aa76f7},
keywords = {Laser induced fluorescence; TALIF; atomic hydrogen; H; dielectric barrier discharges},
language = {eng},
issn = {0963-0252},
journal = {Plasma Sources Science and Technology},
title = {Concentration of atomic hydrogen in a dielectric barrier discharge measured by two-photon absorption fluorescence},
volume = {26},
year = {2017}
}
TY - JOUR
ID - 1385997
AU - Dvořák, Pavel - Talába, Marek - Obrusník, Adam - Jan, Kratzer - Jiří, Dědina
PY - 2017
TI - Concentration of atomic hydrogen in a dielectric barrier discharge measured by two-photon absorption fluorescence
JF - Plasma Sources Science and Technology
VL - 26
IS - 8
SP - nestránkováno
EP - nestránkováno
PB - IOP PUBLISHING LTD
SN - 09630252
KW - Laser induced fluorescence
KW - TALIF
KW - atomic hydrogen
KW - H
KW - dielectric barrier discharges
N2 - Two-photon absorption laser-induced fluorescence (TALIF) was utilized for measuring the concentration of atomic hydrogen in a volume dielectric barrier discharge (DBD) ignited in mixtures of Ar, H2 and O2 at the atmospheric pressure. The method was calibrated by TALIF of krypton diluted in argon at the atmospheric pressure, proving that three-body collisions had negligible effect on quenching of excited krypton atoms. The diagnostic study was complemented with a three-dimensional numerical model of the gas flow and a zero-dimensional model of chemistry in order to better understand the reaction kinetics and identify the key pathways leading to production and destruction of atomic hydrogen. It was determined that the density of atomic hydrogen in Ar - H2 mixtures was in the order of 10^{21} m^{-3} and decreased when oxygen was added into the gas mixture. Spatially resolved measurements and simulations revealed a sharply bordered region with low atomic hydrogen concentration when oxygen was added to the gas mixture. At substoichiometric oxygen/hydrogen ratios, this H-poor region is constricted to an area close to the gas inlet and it is shown that the size of this region is not only influenced by the chemistry but also by the gas flow patterns. Experimentally, it was observed that a decrease of H2 concentration in the feeding Ar - H2 mixture lead to an increase of H production in the DBD.
ER -
DVOŘÁK, Pavel, Marek TALÁBA, Adam OBRUSNÍK, Kratzer JAN and Dědina JIŘÍ. Concentration of atomic hydrogen in a dielectric barrier discharge measured by two-photon absorption fluorescence. \textit{Plasma Sources Science and Technology}. Bristol: IOP PUBLISHING LTD, 2017, vol.~26, No~8, p.~nestránkováno, 13 pp. ISSN~0963-0252. Available from: https://dx.doi.org/10.1088/1361-6595/aa76f7.
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