SHARMA, Brij Mohan, Lisa Emily MELYMUK, Girija K. BHARAT, Petra PŘIBYLOVÁ, Ondřej SÁŇKA, Jana KLÁNOVÁ and Luca NIZZETTO. Spatial gradients of polycyclic aromatic hydrocarbons (PAHs) in air, atmospheric deposition, and surface water of the Ganges River basin. Science of the Total Environment. Amsterdam: Elsevier Science, 2018, vol. 627, June, p. 1495-1504. ISSN 0048-9697. Available from: https://dx.doi.org/10.1016/j.scitotenv.2018.01.262.
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Basic information
Original name Spatial gradients of polycyclic aromatic hydrocarbons (PAHs) in air, atmospheric deposition, and surface water of the Ganges River basin
Authors SHARMA, Brij Mohan (356 India, belonging to the institution), Lisa Emily MELYMUK (124 Canada, belonging to the institution), Girija K. BHARAT (356 India), Petra PŘIBYLOVÁ (203 Czech Republic, belonging to the institution), Ondřej SÁŇKA (203 Czech Republic, belonging to the institution), Jana KLÁNOVÁ (203 Czech Republic, guarantor, belonging to the institution) and Luca NIZZETTO (380 Italy, belonging to the institution).
Edition Science of the Total Environment, Amsterdam, Elsevier Science, 2018, 0048-9697.
Other information
Original language English
Type of outcome Article in a journal
Field of Study 10511 Environmental sciences
Country of publisher Netherlands
Confidentiality degree is not subject to a state or trade secret
WWW URL
Impact factor Impact factor: 5.589
RIV identification code RIV/00216224:14310/18:00104746
Organization unit Faculty of Science
Doi http://dx.doi.org/10.1016/j.scitotenv.2018.01.262
UT WoS 000431848500140
Keywords in English PAHs; Ganges River; Source identification; Urbanization; Health risk assessment
Tags International impact, Reviewed
Changed by Changed by: Mgr. Michaela Hylsová, Ph.D., učo 211937. Changed: 1/12/2018 21:41.
Abstract
Polycyclic aromatic hydrocarbons (PAHs) are ubiquitous semi-volatile organic pollutants. Their environmental occurrence is of global concern as some of them are carcinogens, mutagens, and teratogens. In this study, concentrations and distributions of 16 priority PAHs (Sigma PAHs) were measured in air, atmospheric deposition, and surface water at various locations in Himalayan, Middle, and Lower Reaches of the Ganges River, covering a spatial transect of 2500 km, during two seasons (pre-monsoon and monsoon). The concentration of Sigma PAHs ranged between 2.2 and 182.2 ng m(-3) in air, between 186 and 8810 ng m(-2) day(-1) in atmospheric deposition, and between 0.05 and 65.9 ng L-1 in surface water. Air concentrations were strongly correlated with human population density. In the Middle and Lower Reaches of the Ganges River, atmospheric PAHs were mainly attributed to fossil fuel combustion sources. In the Himalayan Reach the influence of forest fire or biomass combustion was evident during the dry pre-monsoon season. Seasonality in concentrations of PAHs in river water was evident in the Himalayan Reach of the river, as a probable consequence of climate-modulated secondary source intensity (i.e. releases from glacier melting). Seasonality faded in the Middle and Lower Reaches of the Ganges where water contamination is expected to mainly reflect anthropogenic primary sources. Ambient air concentrations were used to calculate the probabilistic incremental lifetime cancer risk (ILCR). It was expectedly found to be higher in the Middle and Lower Reaches compared to the Himalayan Reach. The strong correlation between population density and air concentrations suggests population density may be used as a surrogate variable to assess human health risk in data-sparse regions such as the Ganges River basin.
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CZ.02.1.01/0.0/0.0/16_013/0001761, interní kód MUName: RECETOX RI - OP VVV (Acronym: RECETOX RI)
Investor: Ministry of Education, Youth and Sports of the CR, Priority axis 1: Strengthening capacities for high-quality research
ED2.1.00/19.0382, research and development projectName: CETOCOEN UPgrade
EF15_003/0000469, research and development projectName: Cetocoen Plus
LM2015051, research and development projectName: Centrum pro výzkum toxických látek v prostředí (Acronym: RECETOX RI)
Investor: Ministry of Education, Youth and Sports of the CR
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