| ZHANG, Hui, Luca NIZZETTO, Xinbin FENG, Katrine BORGA, Jonas SOMMAR, Xuewu FU, Hua ZHANG, Gan ZHANG a Thorjorn LARSSEN. Assessing Air-Surface Exchange and Fate of Mercury in a Subtropical Forest Using a Novel Passive Exchange-Meter Device. ENVIRONMENTAL SCIENCE & TECHNOLOGY. WASHINGTON: AMER CHEMICAL SOC, roč. 53, č. 9, s. 4869-4879. ISSN 0013-936X. doi:10.1021/acs.est.8b06343. 2019. |
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@article{1549877,
author = {Zhang, Hui and Nizzetto, Luca and Feng, Xinbin and Borga, Katrine and Sommar, Jonas and Fu, Xuewu and Zhang, Hua and Zhang, Gan and Larssen, Thorjorn},
article_location = {WASHINGTON},
article_number = {9},
doi = {http://dx.doi.org/10.1021/acs.est.8b06343},
keywords = {ATMOSPHERIC MERCURY; LITTER DECOMPOSITION; ELEMENTAL MERCURY; SPATIAL-PATTERNS; GASEOUS MERCURY; ORGANIC-MATTER; STREAM WATER; SOIL; DEPOSITION; EMISSIONS},
language = {eng},
issn = {0013-936X},
journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY},
title = {Assessing Air-Surface Exchange and Fate of Mercury in a Subtropical Forest Using a Novel Passive Exchange-Meter Device},
url = {https://pubs.acs.org/doi/10.1021/acs.est.8b06343},
volume = {53},
year = {2019}
}
TY - JOUR
ID - 1549877
AU - Zhang, Hui - Nizzetto, Luca - Feng, Xinbin - Borga, Katrine - Sommar, Jonas - Fu, Xuewu - Zhang, Hua - Zhang, Gan - Larssen, Thorjorn
PY - 2019
TI - Assessing Air-Surface Exchange and Fate of Mercury in a Subtropical Forest Using a Novel Passive Exchange-Meter Device
JF - ENVIRONMENTAL SCIENCE & TECHNOLOGY
VL - 53
IS - 9
SP - 4869-4879
EP - 4869-4879
PB - AMER CHEMICAL SOC
SN - 0013936X
KW - ATMOSPHERIC MERCURY
KW - LITTER DECOMPOSITION
KW - ELEMENTAL MERCURY
KW - SPATIAL-PATTERNS
KW - GASEOUS MERCURY
KW - ORGANIC-MATTER
KW - STREAM WATER
KW - SOIL
KW - DEPOSITION
KW - EMISSIONS
UR - https://pubs.acs.org/doi/10.1021/acs.est.8b06343
L2 - https://pubs.acs.org/doi/10.1021/acs.est.8b06343
N2 - A novel passive exchange meter (EM) device was developed to assess air-surface exchange and leaching of Hg in a forest floor. Flux measurements were carried out in a subtropical forest ecosystem during a full year. Over 40% of the Hg fixed in fresh forest litter was remobilized in less than 60 days in warm and humid conditions as a response to rapid turnover of labile organic matter (OM). A two-block experiment including understory and clearing showed that losses of Hg covaried with seasonal conditions and was significantly affected by forest coverage. The process controlling the bulk loss of total Hg from the litter was volatilization, which typically represented 76-96% of the loss processes (F-loss). The F-loss ranges were 520-1370 and 165-942 ng m(-2) d(-1) in the understory and clearing, respectively. On a yearly basis, deposition of airborne Hg exceeded total losses by a factor of 2.5 in the clearing and 1.5 in the understory. The vegetation litter in this subtropical forest therefore represented a net sink of atmospheric Hg. This study provided a novel approach to Hg air-soil exchange measurements and further insights on the link between Hg remobilization and OM turnover along with its environmental drivers.
ER -
ZHANG, Hui, Luca NIZZETTO, Xinbin FENG, Katrine BORGA, Jonas SOMMAR, Xuewu FU, Hua ZHANG, Gan ZHANG a Thorjorn LARSSEN. Assessing Air-Surface Exchange and Fate of Mercury in a Subtropical Forest Using a Novel Passive Exchange-Meter Device. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, roč.~53, č.~9, s.~4869-4879. ISSN~0013-936X. doi:10.1021/acs.est.8b06343. 2019.
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