J
2024
Emergent transverse-field Ising model in d4 spin-orbit Mott insulators
CHALOUPKA, Jiří
Basic information
Original name
Emergent transverse-field Ising model in d4 spin-orbit Mott insulators
Authors
CHALOUPKA, Jiří (203 Czech Republic, guarantor, belonging to the institution)
Edition
Physical Review B, College PK, American Physical Society, 2024, 2469-9950
Other information
Type of outcome
Článek v odborném periodiku
Field of Study
10302 Condensed matter physics
Country of publisher
United States of America
Confidentiality degree
není předmětem státního či obchodního tajemství
Impact factor
Impact factor: 3.700 in 2022
Organization unit
Faculty of Science
Keywords in English
Mott insulators; Linear spin wave theory; Exchange interaction; Frustrated magnetism; Magnetic order; Quantum phase transitions; Spin dynamics
Tags
International impact, Reviewed
V originále
Mott-insulating transition metal oxides containing t<SUB>2</SUB><SUP>g 4</SUP> ions with strong spin-orbit coupling were recently demonstrated to display unusual magnetism due to a dynamical mixing of the low-energy multiplet states via exchange processes. Here we derive exchange interactions in the situation where a tetragonal or trigonal crystal field selects a single relevant excited state on top of the singlet ionic ground state, producing an effective spin-1/2 . We show that these moments universally obey antiferromagnetic transverse-field Ising model (TFIM) with an intrinsic transverse field generated by the splitting of the two ionic singlets. Using Ru<SUP>4 +</SUP> as a example ion, we provide quantitative estimates of the exchange and illustrate the emergent TFIM physics based on phase diagrams and excitation spectra obtained for several 2D lattices—square, honeycomb, as well as for the frustrated triangular lattice.
Links
GA22-28797S, research and development project | Name: Pohybliví nositelé náboje v exotických magnetech se spin-orbitálním propletením | Investor: Czech Science Foundation |
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Displayed: 14/11/2024 07:48