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@article{1163807, author = {Lohmann, Rainer and Klánová, Jana and Kukučka, Petr and Yonis, Shifra and Bollinger, Kevyn}, article_location = {WASHINGTON}, article_number = {24}, doi = {http://dx.doi.org/10.1021/es403494b}, keywords = {POLYBROMINATED DIPHENYL ETHERS; PERSISTENT ORGANIC POLLUTANTS; POLYCHLORINATED-BIPHENYLS; PHYSICOCHEMICAL PROPERTIES; PERFLUORINATED ACIDS; ENVIRONMENTAL FATE; SURFACE SEAWATER; DRY DEPOSITION; AIR-WATER; PCBS}, language = {eng}, issn = {0013-936X}, journal = {ENVIRONMENTAL SCIENCE andTECHNOLOGY}, title = {Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean}, volume = {47}, year = {2013} }
TY - JOUR ID - 1163807 AU - Lohmann, Rainer - Klánová, Jana - Kukučka, Petr - Yonis, Shifra - Bollinger, Kevyn PY - 2013 TI - Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean JF - ENVIRONMENTAL SCIENCE andTECHNOLOGY VL - 47 IS - 24 SP - 13967-13975 EP - 13967-13975 PB - AMER CHEMICAL SOC SN - 0013936X KW - POLYBROMINATED DIPHENYL ETHERS KW - PERSISTENT ORGANIC POLLUTANTS KW - POLYCHLORINATED-BIPHENYLS KW - PHYSICOCHEMICAL PROPERTIES KW - PERFLUORINATED ACIDS KW - ENVIRONMENTAL FATE KW - SURFACE SEAWATER KW - DRY DEPOSITION KW - AIR-WATER KW - PCBS N2 - Little is known about the fate of polybrominated diphenylethers (PBDEs) across the Oceans. Air and water were sampled using both active and passive polyethylene samplers on an east-west transect across the tropical Atlantic Ocean in 2009 and analyzed for PBDEs. Typical particle-bound concentrations of PBDEs in the surface water were low, at <1 pg L-1. Truly dissolved concentrations from passive samplers were similar to 40.5 pg L-1 for BDE 47 and around 0.1 pg L-1 for BDEs 28, 99, and 100 (results from active samples were compromised). In the atmosphere, particle-bound BDE 209 dominated overall concentrations (median 1.2 pg m(-3)), followed by BDE 99 (0.13 pg m(-3)). Gas-phase concentrations based on passive samplers were 1-8 pg m(-3) for BDE 47 and <= 4 pg m(-3) for BDE 99. Net air-water exchange gradients strongly favored gas-phase deposition of PBDEs into the water. Net gas-phase deposition fluxes ranged from tens of pg m(-2) day(-1) for BDEs 28 and 85 to around 1 ng m(-2) day(-1) for BDE 47, 99, and 209. Settling fluxes of particle-bound PBDEs in the atmosphere and surface water were around 50 pg m(-2) day(-1) for BDE 47 and <10 pg m(-2) day(-1) for the other congeners. ER -
LOHMANN, Rainer, Jana KLÁNOVÁ, Petr KUKUČKA, Shifra YONIS a Kevyn BOLLINGER. Concentrations, Fluxes, and Residence Time of PBDEs Across the Tropical Atlantic Ocean. \textit{ENVIRONMENTAL SCIENCE andTECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2013, roč.~47, č.~24, s.~13967-13975. ISSN~0013-936X. Dostupné z: https://dx.doi.org/10.1021/es403494b.
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