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@article{1298031,
author = {Banerjee, Rupak and Novák, Jiří and Frank, Christian and Girleanu, Maria and Ersen, Olivier and Brinkmann, Martin and Anger, Falk and Lorch, Christian and Dieterle, Johannes and Gerlach, Alexander and Drnec, Jakub and Yu, Sun and Schreiber, Frank},
article_location = {Washington D.C.},
article_number = {9},
doi = {http://dx.doi.org/10.1021/acs.jpcc.5b00480},
keywords = {hybrid thin films; organic semiconductors; nano-particles; spin-casting; organic molecular beam-deposition; structure; morphology; GISAXS; GIXRD; X-ray reflectivity; TEM; AFM; photoluminiscence},
language = {eng},
issn = {1932-7447},
journal = {JOURNAL OF PHYSICAL CHEMISTRY C},
title = {Structure and Morphology of Organic Semiconductor-Nanoparticle Hybrids Prepared by Soft Deposition},
url = {http://pubs.acs.org/doi/abs/10.1021/acs.jpcc.5b00480},
volume = {119},
year = {2015}
}
TY - JOUR
ID - 1298031
AU - Banerjee, Rupak - Novák, Jiří - Frank, Christian - Girleanu, Maria - Ersen, Olivier - Brinkmann, Martin - Anger, Falk - Lorch, Christian - Dieterle, Johannes - Gerlach, Alexander - Drnec, Jakub - Yu, Sun - Schreiber, Frank
PY - 2015
TI - Structure and Morphology of Organic Semiconductor-Nanoparticle Hybrids Prepared by Soft Deposition
JF - JOURNAL OF PHYSICAL CHEMISTRY C
VL - 119
IS - 9
SP - 5225-5237
EP - 5225-5237
PB - American Chemical Society
SN - 19327447
KW - hybrid thin films
KW - organic semiconductors
KW - nano-particles
KW - spin-casting
KW - organic molecular beam-deposition
KW - structure
KW - morphology
KW - GISAXS
KW - GIXRD
KW - X-ray reflectivity
KW - TEM
KW - AFM
KW - photoluminiscence
UR - http://pubs.acs.org/doi/abs/10.1021/acs.jpcc.5b00480
L2 - http://pubs.acs.org/doi/abs/10.1021/acs.jpcc.5b00480
N2 - We present an extensive structural analysis of hybrid architectures prepared by the soft incorporation of gold nanoparticles (AuNPs) within an organic semiconductor matrix of diindenoperylene (DIP). Such soft or noninvasive deposition of nanoparticles within organic semiconducting host matrices not only minimizes the influence of the deposition process on the order and properties of the organic host molecules, but also offers additional control in the process of incorporation. The hybrid structures were characterized by X-ray scattering techniques including grazing incidence small angle X-ray scattering (GISAXS), grazing incidence X-ray diffraction (GIXD), X-ray reflectivity (XRR), and complemented by atomic force microscopy (AFM), photoluminescence (PL) spectroscopy, and transmission electron microscopy (TEM) measurements. We show that different strategies of incorporating the nanoparticles in the host matrix lead to drastically different structure and morphologies. Particularly remarkable is the morphological change observed in the matrix of DIP as well as the AuNPs due to the influence of organic solvents, as evidenced by TEM tomography measurements, which revealed the exact location of the AuNPs within the organic host. It is also demonstrated that AuNPs can be successfully used as tunable templates for the growth of the organic semiconductors with desired island sizes and distances.
ER -
BANERJEE, Rupak, Jiří NOVÁK, Christian FRANK, Maria GIRLEANU, Olivier ERSEN, Martin BRINKMANN, Falk ANGER, Christian LORCH, Johannes DIETERLE, Alexander GERLACH, Jakub DRNEC, Sun YU and Frank SCHREIBER. Structure and Morphology of Organic Semiconductor-Nanoparticle Hybrids Prepared by Soft Deposition. \textit{JOURNAL OF PHYSICAL CHEMISTRY C}. Washington D.C.: American Chemical Society, 2015, vol.~119, No~9, p.~5225-5237. ISSN~1932-7447. Available from: https://dx.doi.org/10.1021/acs.jpcc.5b00480.
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