Direct evidence for dominant bond-directional interactions in a
honeycomb lattice iridate Na2IrO3

J 2015

Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3

CHUN, Sae Hwan, Jong-Woo KIM, Jungho KIM, H. ZHENG, Constantinos C STOUMPOS et. al.

Základní údaje

Originální název

Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3

Název česky

Přímý důkaz dominantních vazebně-směrových interakcí v iridátu Na2IrO3 s voštinovou mřížkou

Autoři

CHUN, Sae Hwan (410 Korejská republika), Jong-Woo KIM (410 Korejská republika), Jungho KIM (410 Korejská republika), H. ZHENG (156 Čína), Constantinos C STOUMPOS (840 Spojené státy), C.D. MALLIAKAS (840 Spojené státy), J.F. MITCHELL (840 Spojené státy), Kavita MEHLAWAT (356 Indie), Yogesh SINGH (356 Indie), Y. CHOI (410 Korejská republika), T. GOG (840 Spojené státy), A. AL-ZEIN (250 Francie), M. Moretti SALA (380 Itálie), M. KRISCH (276 Německo), Jiří CHALOUPKA (203 Česká republika, garant, domácí), George JACKELI (268 Gruzie), Giniyat KHALIULLIN (643 Rusko) a B.J. KIM (410 Korejská republika)

Vydání

Nature Physics, London, Nature Publishing Group, 2015, 1745-2473

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10302 Condensed matter physics

Stát vydavatele

Velká Británie a Severní Irsko

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 18.791

Kód RIV

RIV/00216224:14740/15:00086048

Organizační jednotka

Středoevropský technologický institut

DOI

http://dx.doi.org/10.1038/NPHYS3322

UT WoS

000355552200010

Klíčová slova česky

spinové interakce; frustrovaný magnetismus; iridáty; spinové modely

Klíčová slova anglicky

spin interactions; frustrated magnetism; iridates; spin models

Štítky

podil, rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 18. 3. 2016 10:52, doc. Mgr. Jiří Chaloupka, Ph.D.

Anotace

V originále

Heisenberg interactions are ubiquitous in magnetic materials and play a central role in modelling and designing quantum magnets. Bond-directional interactions offer a novel alternative to Heisenberg exchange and provide the building blocks of the Kitaev model, which has a quantum spin liquid as its exact ground state. Honeycomb iridates, A2IrO3 (A = Na, Li), offer potential realizations of the Kitaev magnetic exchange coupling, and their reported magnetic behaviour may be interpreted within the Kitaev framework. However, the extent of their relevance to the Kitaev model remains unclear, as evidence for bond-directional interactions has so far been indirect. Herewe present direct evidence for dominant bond-directional interactions in antiferromagnetic Na2IrO3 and show that they lead to strong magnetic frustration. Diffuse magnetic X-ray scattering reveals broken spin-rotational symmetry even above the Neel temperature, with the three spin components exhibiting short-range correlations along distinct crystallographic directions. This spin- and real-space entanglement directly uncovers the bond-directional nature of these interactions, thus providing a direct connection between honeycomb iridates and Kitaev physics.

Návaznosti

ED1.1.00/02.0068, projekt VaV

Název: CEITEC - central european institute of technology

286154, interní kód MU

Název: SYLICA - Synergies of Life and Material Sciences to Create a New Future (Akronym: SYLICA)

Investor: Evropská unie, SYLICA - Synergies of Life and Material Sciences to Create a New Future, Kapacity

Citovat

CHUN, Sae Hwan, Jong-Woo KIM, Jungho KIM, H. ZHENG, Constantinos C STOUMPOS, C.D. MALLIAKAS, J.F. MITCHELL, Kavita MEHLAWAT, Yogesh SINGH, Y. CHOI, T. GOG, A. AL-ZEIN, M. Moretti SALA, M. KRISCH, Jiří CHALOUPKA, George JACKELI, Giniyat KHALIULLIN a B.J. KIM. Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3. Nature Physics. London: Nature Publishing Group, 2015, roč. 11, č. 6, s. 462-467. ISSN 1745-2473. Dostupné z: https://dx.doi.org/10.1038/NPHYS3322.

@article{1331271,
   author = {Chun, Sae Hwan and Kim, JongandWoo and Kim, Jungho and Zheng, H. and Stoumpos, Constantinos C and Malliakas, C.D. and Mitchell, J.F. and Mehlawat, Kavita and Singh, Yogesh and Choi, Y. and Gog, T. and AlandZein, A. and Sala, M. Moretti and Krisch, M. and Chaloupka, Jiří and Jackeli, George and Khaliullin, Giniyat and Kim, B.J.},
   article_location = {London},
   article_number = {6},
   doi = {http://dx.doi.org/10.1038/NPHYS3322},
   keywords = {spin interactions; frustrated magnetism; iridates; spin models},
   language = {eng},
   issn = {1745-2473},
   journal = {Nature Physics},
   title = {Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3},
   url = {http://www.nature.com/nphys/journal/v11/n6/full/nphys3322.html},
   volume = {11},
   year = {2015}
}

TY  - JOUR
ID  - 1331271
AU  - Chun, Sae Hwan - Kim, Jong-Woo - Kim, Jungho - Zheng, H. - Stoumpos, Constantinos C - Malliakas, C.D. - Mitchell, J.F. - Mehlawat, Kavita - Singh, Yogesh - Choi, Y. - Gog, T. - Al-Zein, A. - Sala, M. Moretti - Krisch, M. - Chaloupka, Jiří - Jackeli, George - Khaliullin, Giniyat - Kim, B.J.
PY  - 2015
TI  - Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3
JF  - Nature Physics
VL  - 11
IS  - 6
SP  - 462-467
EP  - 462-467
PB  - Nature Publishing Group
SN  - 17452473
KW  - spin interactions
KW  - frustrated magnetism
KW  - iridates
KW  - spin models
UR  - http://www.nature.com/nphys/journal/v11/n6/full/nphys3322.html
L2  - http://www.nature.com/nphys/journal/v11/n6/full/nphys3322.html
N2  - Heisenberg interactions are ubiquitous in magnetic materials and play a central role in modelling and designing quantum magnets. Bond-directional interactions offer a novel alternative to Heisenberg exchange and provide the building blocks of the Kitaev model, which has a quantum spin liquid as its exact ground state. Honeycomb iridates, A2IrO3 (A = Na, Li), offer potential realizations of the Kitaev magnetic exchange coupling, and their reported magnetic behaviour may be interpreted within the Kitaev framework. However, the extent of their relevance to the Kitaev model remains unclear, as evidence for bond-directional interactions has so far been indirect. Herewe present direct evidence for dominant bond-directional interactions in antiferromagnetic Na2IrO3 and show that they lead to strong magnetic frustration. Diffuse magnetic X-ray scattering reveals broken spin-rotational symmetry even above the Neel temperature, with the three spin components exhibiting short-range correlations along distinct crystallographic directions. This spin- and real-space entanglement directly uncovers the bond-directional nature of these interactions, thus providing a direct connection between honeycomb iridates and Kitaev physics.
ER  -

CHUN, Sae Hwan, Jong-Woo KIM, Jungho KIM, H. ZHENG, Constantinos C STOUMPOS, C.D. MALLIAKAS, J.F. MITCHELL, Kavita MEHLAWAT, Yogesh SINGH, Y. CHOI, T. GOG, A. AL-ZEIN, M. Moretti SALA, M. KRISCH, Jiří CHALOUPKA, George JACKELI, Giniyat KHALIULLIN a B.J. KIM. Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3. \textit{Nature Physics}. London: Nature Publishing Group, 2015, roč.~11, č.~6, s.~462-467. ISSN~1745-2473. Dostupné z: https://dx.doi.org/10.1038/NPHYS3322.

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