Laser Ablation Synthesis of Gold Selenides by Using a Mass
Spectrometer as a Synthesizer: Laser Desorption Ionization
Time-of-Flight Mass Spectrometry

J 2016

Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry

PROKEŠ, Lubomír, Pavel KUBÁČEK, Eladia Maria PEÑA-MÉNDEZ, Filippo AMATO, Jose Elias CONDE et. al.

Základní údaje

Originální název

Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry

Autoři

PROKEŠ, Lubomír (203 Česká republika, domácí), Pavel KUBÁČEK (203 Česká republika, domácí), Eladia Maria PEÑA-MÉNDEZ (724 Španělsko), Filippo AMATO (380 Itálie, domácí), Jose Elias CONDE (724 Španělsko), Milan ALBERTI (203 Česká republika, garant, domácí) a Josef HAVEL (203 Česká republika, domácí)

Vydání

Chemistry – A European Journal, Weinheim, Wiley, 2016, 0947-6539

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10406 Analytical chemistry

Stát vydavatele

Německo

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 5.317

Kód RIV

RIV/00216224:14310/16:00088087

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1002/chem.201600160

UT WoS

000382918700025

Klíčová slova anglicky

laser ablation synthesis; gold selenides; LDI-TOF; clusters; mass spectrometry

Štítky

AKR, rivok

Změněno: 26. 4. 2017 22:11, Ing. Andrea Mikešková

Anotace

V originále

Methods for the rapid construction of new chemical motifs have the potential to accelerate the development of nanoscience. The synthesis of new chemical entities by laser ablation has been systematically demonstrated by using mixtures of gold and selenium. The compounds generated are detected by time-of-flight mass spectrometry and, for selected compounds, the structure is investigated by using density functional theory optimization. In total, 67 new gold selenide clusters have been synthesized, demonstrating an unsuspected richness in gold chemistry. Chemical species generated in the gas phase might inspire new routes for the synthesis of novel compounds in the solid state.

Návaznosti

ED2.1.00/03.0086, projekt VaV

Název: Regionální VaV centrum pro nízkonákladové plazmové a nanotechnologické povrchové úpravy

GA13-05082S, projekt VaV

Název: Analýza a aplikace plazmatických procesů pro přípravu tenkých vrstev amorfních chalkogenidů

Investor: Grantová agentura ČR, Analýza a aplikace plazmatických procesů pro přípravu tenkých vrstev amorfních chalkogenidů

LO1411, projekt VaV

Název: Rozvoj centra pro nízkonákladové plazmové a nanotechnologické povrchové úpravy (Akronym: CEPLANT plus)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Rozvoj centra pro nízkonákladové plazmové a nanotechnologické povrchové úpravy

Citovat

PROKEŠ, Lubomír, Pavel KUBÁČEK, Eladia Maria PEÑA-MÉNDEZ, Filippo AMATO, Jose Elias CONDE, Milan ALBERTI a Josef HAVEL. Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry. Chemistry – A European Journal. Weinheim: Wiley, 2016, roč. 22, č. 32, s. 11261-11268. ISSN 0947-6539. Dostupné z: https://dx.doi.org/10.1002/chem.201600160.

@article{1352176,
   author = {Prokeš, Lubomír and Kubáček, Pavel and PeñaandMéndez, Eladia Maria and Amato, Filippo and Conde, Jose Elias and Alberti, Milan and Havel, Josef},
   article_location = {Weinheim},
   article_number = {32},
   doi = {http://dx.doi.org/10.1002/chem.201600160},
   keywords = {laser ablation synthesis; gold selenides; LDI-TOF; clusters; mass spectrometry},
   language = {eng},
   issn = {0947-6539},
   journal = {Chemistry – A European Journal},
   title = {Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry},
   url = {http://onlinelibrary.wiley.com/doi/10.1002/chem.201600160/full},
   volume = {22},
   year = {2016}
}

TY  - JOUR
ID  - 1352176
AU  - Prokeš, Lubomír - Kubáček, Pavel - Peña-Méndez, Eladia Maria - Amato, Filippo - Conde, Jose Elias - Alberti, Milan - Havel, Josef
PY  - 2016
TI  - Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry
JF  - Chemistry – A European Journal
VL  - 22
IS  - 32
SP  - 11261-11268
EP  - 11261-11268
PB  - Wiley
SN  - 09476539
KW  - laser ablation synthesis
KW  - gold selenides
KW  - LDI-TOF
KW  - clusters
KW  - mass spectrometry
UR  - http://onlinelibrary.wiley.com/doi/10.1002/chem.201600160/full
N2  - Methods for the rapid construction of new chemical motifs have the potential to accelerate the development of nanoscience. The synthesis of new chemical entities by laser ablation has been systematically demonstrated by using mixtures of gold and selenium. The compounds generated are detected by time-of-flight mass spectrometry and, for selected compounds, the structure is investigated by using density functional theory optimization. In total, 67 new gold selenide clusters have been synthesized, demonstrating an unsuspected richness in gold chemistry. Chemical species generated in the gas phase might inspire new routes for the synthesis of novel compounds in the solid state.
ER  -

PROKEŠ, Lubomír, Pavel KUBÁČEK, Eladia Maria PEÑA-MÉNDEZ, Filippo AMATO, Jose Elias CONDE, Milan ALBERTI a Josef HAVEL. Laser Ablation Synthesis of Gold Selenides by Using a Mass Spectrometer as a Synthesizer: Laser Desorption Ionization Time-of-Flight Mass Spectrometry. \textit{Chemistry – A European Journal}. Weinheim: Wiley, 2016, roč.~22, č.~32, s.~11261-11268. ISSN~0947-6539. Dostupné z: https://dx.doi.org/10.1002/chem.201600160.

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