| ŠPONEROVÁ, Judit, Rafal Kazimierz SZABLA, Robert W. GORA, A. Marco SAITTA, Fabio PIETRUCCI, Franz SAIJA, Ernesto DI MAURO, Raffaele SALADINO, Martin FERUS, Svatopluk CIVIŠ a Jiří ŠPONER. Prebiotic synthesis of nucleic acids and their building blocks at the atomic level - merging models and mechanisms from advanced computations and experiments. Physical Chemistry Chemical Physics. Cambridge: Royal Society of Chemistry, 2016, roč. 18, č. 30, s. 20047-20066. ISSN 1463-9076. Dostupné z: https://dx.doi.org/10.1039/c6cp00670a. |
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@article{1356116,
author = {Šponerová, Judit and Szabla, Rafal Kazimierz and Gora, Robert W. and Saitta, A. Marco and Pietrucci, Fabio and Saija, Franz and Di Mauro, Ernesto and Saladino, Raffaele and Ferus, Martin and Civiš, Svatopluk and Šponer, Jiří},
article_location = {Cambridge},
article_number = {30},
doi = {http://dx.doi.org/10.1039/c6cp00670a},
keywords = {EXCITED-STATE DYNAMICS; DRIVEN PROTON-TRANSFER; HIGH-POWER LASER; INDUCED DIELECTRIC-BREAKDOWN; TEMPLATE-DIRECTED SYNTHESIS; CLASSICAL DRUDE OSCILLATOR; DENSITY-FUNCTIONAL THEORY; POLARIZABLE FORCE-FIELD; SIGMA-ASTERISK STATES; HIGH-ENERGY CHEMISTRY},
language = {eng},
issn = {1463-9076},
journal = {Physical Chemistry Chemical Physics},
title = {Prebiotic synthesis of nucleic acids and their building blocks at the atomic level - merging models and mechanisms from advanced computations and experiments},
url = {http://pubs.rsc.org/en/content/articlepdf/2016/cp/c6cp00670a},
volume = {18},
year = {2016}
}
TY - JOUR
ID - 1356116
AU - Šponerová, Judit - Szabla, Rafal Kazimierz - Gora, Robert W. - Saitta, A. Marco - Pietrucci, Fabio - Saija, Franz - Di Mauro, Ernesto - Saladino, Raffaele - Ferus, Martin - Civiš, Svatopluk - Šponer, Jiří
PY - 2016
TI - Prebiotic synthesis of nucleic acids and their building blocks at the atomic level - merging models and mechanisms from advanced computations and experiments
JF - Physical Chemistry Chemical Physics
VL - 18
IS - 30
SP - 20047-20066
EP - 20047-20066
PB - Royal Society of Chemistry
SN - 14639076
KW - EXCITED-STATE DYNAMICS
KW - DRIVEN PROTON-TRANSFER
KW - HIGH-POWER LASER
KW - INDUCED DIELECTRIC-BREAKDOWN
KW - TEMPLATE-DIRECTED SYNTHESIS
KW - CLASSICAL DRUDE OSCILLATOR
KW - DENSITY-FUNCTIONAL THEORY
KW - POLARIZABLE FORCE-FIELD
KW - SIGMA-ASTERISK STATES
KW - HIGH-ENERGY CHEMISTRY
UR - http://pubs.rsc.org/en/content/articlepdf/2016/cp/c6cp00670a
L2 - http://pubs.rsc.org/en/content/articlepdf/2016/cp/c6cp00670a
N2 - The origin of life on Earth is one of the most fascinating questions of contemporary science. Extensive research in the past decades furnished diverse experimental proposals for the emergence of first informational polymers that could form the basis of the early terrestrial life. Side by side with the experiments, the fast development of modern computational chemistry methods during the last 20 years facilitated the use of in silico modelling tools to complement the experiments. Modern computations can provide unique atomic-level insights into the structural and electronic aspects as well as the energetics of key prebiotic chemical reactions. Many of these insights are not directly obtainable from the experimental techniques and the computations are thus becoming indispensable for proper interpretation of many experiments and for qualified predictions. This review illustrates the synergy between experiment and theory in the origin of life research focusing on the prebiotic synthesis of various nucleic acid building blocks and on the self-assembly of nucleotides leading to the first functional oligonucleotides.
ER -
ŠPONEROVÁ, Judit, Rafal Kazimierz SZABLA, Robert W. GORA, A. Marco SAITTA, Fabio PIETRUCCI, Franz SAIJA, Ernesto DI MAURO, Raffaele SALADINO, Martin FERUS, Svatopluk CIVIŠ a Jiří ŠPONER. Prebiotic synthesis of nucleic acids and their building blocks at the atomic level - merging models and mechanisms from advanced computations and experiments. \textit{Physical Chemistry Chemical Physics}. Cambridge: Royal Society of Chemistry, 2016, roč.~18, č.~30, s.~20047-20066. ISSN~1463-9076. Dostupné z: https://dx.doi.org/10.1039/c6cp00670a.
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