Diurnal Variations of Air-Soil Exchange of Semivolatile Organic
Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European
Receptor Area

J 2016

Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area

DEGRENDELE, Celine, Ondřej AUDY, Jakub HOFMAN, Jiří KUCERIK, Petr KUKUČKA et. al.

Základní údaje

Originální název

Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area

Autoři

DEGRENDELE, Celine (250 Francie), Ondřej AUDY (203 Česká republika, domácí), Jakub HOFMAN (203 Česká republika, domácí), Jiří KUCERIK (203 Česká republika), Petr KUKUČKA (203 Česká republika, domácí), Marie Daniëlle MULDER (528 Nizozemské království, domácí), Petra PŘIBYLOVÁ (203 Česká republika, domácí), Roman PROKEŠ (203 Česká republika, domácí), Milan SÁŇKA (203 Česká republika, domácí), Gabriele E. SCHAUMANN (276 Německo) a Gerhard LAMMEL (276 Německo, garant, domácí)

Vydání

ENVIRONMENTAL SCIENCE & TECHNOLOGY, WASHINGTON, AMER CHEMICAL SOC, 2016, 0013-936X

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

30304 Public and environmental health

Stát vydavatele

Spojené státy

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 6.198

Kód RIV

RIV/00216224:14310/16:00088654

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1021/acs.est.5b05671

UT WoS

000374707100016

Klíčová slova anglicky

POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; CENTRAL TIBETAN PLATEAU; ORGANOCHLORINE PESTICIDES; POLYCHLORINATED-BIPHENYLS; PARTITION-COEFFICIENTS; SURFACE SOIL; BLACK CARBON; SPATIAL-DISTRIBUTION; ATMOSPHERIC CONCENTRATIONS

Štítky

AKR, rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 2. 3. 2017 14:15, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

Concentrations of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), organochlorine pesticides (OCPs), and polybrominated diphenyl ethers (PBDEs) in air and soil, their fugacities, and the experimental soil-air partitioning coefficient (K-SA) were determined at two background sites in the Gt. Hungarian Plain in August 2013. The concentrations of the semivolatile organic compounds (SOCs) in the soil were not correlated with the organic carbon content but with two indirect parameters of mineralization and aromaticity, suggesting that soil organic matter quality is an important parameter affecting the sorption of SOCs onto soils. Predictions based on the assumption that absorption is the dominant process were in good agreement with the measurements for PAHs, OCPs, and the low chlorinated PCBs. In general, soils were found to be a source of PAHs, high chlorinated PCBs, the majority of OCPs and PBDEs, and a sink for the low chlorinated PCBs and gamma-hexachlorocyclohexane. Diurnal variations in the direction of the soil-air exchange were found for two compounds (i.e., pentachlorobenzene and p,p'-dichlorodiphenyldichloroethane), with volatilization during the day and deposition in the night. The concentrations of most SOCs in the near-ground atmosphere were dominated by revolatilization from the soil.

Návaznosti

GAP503/11/1230, projekt VaV

Název: Perzistentní organické polutanty v atmosférických aerosolech: Procesy, které ovlivňují dálkový transport v Evropě.

Investor: Grantová agentura ČR, Perzistentní organické polutanty v atmosférických aerosolech: procesy, které ovlivňují dálkový transport v Evropě

LM2015051, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Výzkumná infrastruktura RECETOX

LO1214, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Centrum pro výzkum toxických látek v prostředí

Citovat

DEGRENDELE, Celine, Ondřej AUDY, Jakub HOFMAN, Jiří KUCERIK, Petr KUKUČKA, Marie Daniëlle MULDER, Petra PŘIBYLOVÁ, Roman PROKEŠ, Milan SÁŇKA, Gabriele E. SCHAUMANN a Gerhard LAMMEL. Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area. ENVIRONMENTAL SCIENCE & TECHNOLOGY. WASHINGTON: AMER CHEMICAL SOC, 2016, roč. 50, č. 8, s. 4278-4288. ISSN 0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.5b05671.

@article{1371893,
   author = {Degrendele, Celine and Audy, Ondřej and Hofman, Jakub and Kucerik, Jiří and Kukučka, Petr and Mulder, Marie Daniëlle and Přibylová, Petra and Prokeš, Roman and Sáňka, Milan and Schaumann, Gabriele E. and Lammel, Gerhard},
   article_location = {WASHINGTON},
   article_number = {8},
   doi = {http://dx.doi.org/10.1021/acs.est.5b05671},
   keywords = {POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; CENTRAL TIBETAN PLATEAU; ORGANOCHLORINE PESTICIDES; POLYCHLORINATED-BIPHENYLS; PARTITION-COEFFICIENTS; SURFACE SOIL; BLACK CARBON; SPATIAL-DISTRIBUTION; ATMOSPHERIC CONCENTRATIONS},
   language = {eng},
   issn = {0013-936X},
   journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY},
   title = {Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area},
   url = {http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671},
   volume = {50},
   year = {2016}
}

TY  - JOUR
ID  - 1371893
AU  - Degrendele, Celine - Audy, Ondřej - Hofman, Jakub - Kucerik, Jiří - Kukučka, Petr - Mulder, Marie Daniëlle - Přibylová, Petra - Prokeš, Roman - Sáňka, Milan - Schaumann, Gabriele E. - Lammel, Gerhard
PY  - 2016
TI  - Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area
JF  - ENVIRONMENTAL SCIENCE & TECHNOLOGY
VL  - 50
IS  - 8
SP  - 4278-4288
EP  - 4278-4288
PB  - AMER CHEMICAL SOC
SN  - 0013936X
KW  - POLYCYCLIC AROMATIC-HYDROCARBONS
KW  - POLYBROMINATED DIPHENYL ETHERS
KW  - CENTRAL TIBETAN PLATEAU
KW  - ORGANOCHLORINE PESTICIDES
KW  - POLYCHLORINATED-BIPHENYLS
KW  - PARTITION-COEFFICIENTS
KW  - SURFACE SOIL
KW  - BLACK CARBON
KW  - SPATIAL-DISTRIBUTION
KW  - ATMOSPHERIC CONCENTRATIONS
UR  - http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671
L2  - http://pubs.acs.org/doi/abs/10.1021/acs.est.5b05671
N2  - Concentrations of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), organochlorine pesticides (OCPs), and polybrominated diphenyl ethers (PBDEs) in air and soil, their fugacities, and the experimental soil-air partitioning coefficient (K-SA) were determined at two background sites in the Gt. Hungarian Plain in August 2013. The concentrations of the semivolatile organic compounds (SOCs) in the soil were not correlated with the organic carbon content but with two indirect parameters of mineralization and aromaticity, suggesting that soil organic matter quality is an important parameter affecting the sorption of SOCs onto soils. Predictions based on the assumption that absorption is the dominant process were in good agreement with the measurements for PAHs, OCPs, and the low chlorinated PCBs. In general, soils were found to be a source of PAHs, high chlorinated PCBs, the majority of OCPs and PBDEs, and a sink for the low chlorinated PCBs and gamma-hexachlorocyclohexane. Diurnal variations in the direction of the soil-air exchange were found for two compounds (i.e., pentachlorobenzene and p,p'-dichlorodiphenyldichloroethane), with volatilization during the day and deposition in the night. The concentrations of most SOCs in the near-ground atmosphere were dominated by revolatilization from the soil.
ER  -

DEGRENDELE, Celine, Ondřej AUDY, Jakub HOFMAN, Jiří KUCERIK, Petr KUKUČKA, Marie Dani$\backslash$''elle MULDER, Petra PŘIBYLOVÁ, Roman PROKEŠ, Milan SÁŇKA, Gabriele E. SCHAUMANN a Gerhard LAMMEL. Diurnal Variations of Air-Soil Exchange of Semivolatile Organic Compounds (PAHs, PCBs, OCPs, and PBDEs) in a Central European Receptor Area. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2016, roč.~50, č.~8, s.~4278-4288. ISSN~0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.5b05671.

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