Assessment of a novel device for onsite integrative
large-volume solid phase extraction of water samples to enable
a comprehensive chemical and effect-based analysis

J 2017

Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis

SCHULZE, Tobias, Marijan AHEL, Joerg AHLHEIM, Selim AIT-AISSA, Francois BRION et. al.

Základní údaje

Originální název

Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis

Autoři

SCHULZE, Tobias (276 Německo), Marijan AHEL (191 Chorvatsko), Joerg AHLHEIM, Selim AIT-AISSA (250 Francie), Francois BRION (250 Francie), Carolina DI PAOLO (276 Německo), Jean FROMENT (578 Norsko), Anita O. HIDASI (756 Švýcarsko), Juliane HOLLENDER (756 Švýcarsko), Henner HOLLERT (276 Německo), Meng HU (276 Německo), Anett KLOLSS (276 Německo), Sanja KOPRIVICA (191 Chorvatsko), Martin KRAUSS (276 Německo), Melis MUZ (276 Německo), Peter OSWALD (703 Slovensko), Margit PETRE (276 Německo), Jennifer E. SCHOLLEE (756 Švýcarsko), Thomas-Benjamin SEILER (276 Německo), Ying SHAO (276 Německo), Jaroslav SLOBODNÍK (703 Slovensko), Manoj SONAVANE (250 Francie), Marc J. F. SUTER (756 Švýcarsko), Knut Erik TOLLEFSEN (578 Norsko), Zuzana TOUŠOVÁ (203 Česká republika, garant, domácí), Karl-Heinz WALZ (276 Německo) a Werner BRACK (276 Německo)

Vydání

Science of the Total Environment, Elsevier, 2017, 0048-9697

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Nizozemské království

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 4.610

Kód RIV

RIV/00216224:14310/17:00120354

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1016/j.scitotenv.2016.12.140

UT WoS

000394635300033

Klíčová slova anglicky

Automated water sampler; Chemical analysis; Bioassay analysis; Effect-based analysis; Applicability domain; Large-volume solid phase extraction; LVSPE

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 2. 11. 2021 11:25, Mgr. Marie Šípková, DiS.

Anotace

V originále

The implementation of targeted and nontargeted chemical screening analysis in combination with in vitro and organism-level bioassays is a prerequisite for a more holistic monitoring of water quality in the future. For chemical analysis, little or no sample enrichment is often sufficient, while bioanalysis often requires larger sample volumes at a certain enrichment factor for conducting comprehensive bioassays on different endpoints or furthereffect-directed analysis (EDA). To avoid logistic and technical issues related to the storage and transport of large volumes of water, sampling would benefit greatly from onsite extraction. This study presents a novel onsite large volume solid phase extraction (LVSPE) device tailored to fulfill the requirements for the successful effect-based and chemical screening of water resources and complies with available international standards for automated sampling devices. Laboratory recovery experiments using 251 organic compounds in the log D range from -3.6 to 9.4 (at pH 7.0) spiked into pristine water resulted in acceptable recoveries and from 60 to 123% for 159 out of 251 substances. Within a European-wide demonstration program, the LVSPE was able to enrich compounds in concentration ranges over three orders of magnitude (1 ng L-1 to 2400 ng L-1). It was possible to discriminate responsive samples from samples with no or only low effects in a set of six different bioassays "( i.e. acetylcholinesterase and algal growth inhibition, androgenicity, estrogenicity, fish embryo toxicity, glucocorticoid activity). The LVSPE thus proved applicable for onsite extraction of sufficient amounts of water to investigate water quality thoroughly by means of chemical analysis and effect-based tools without the common limitations due to small sample volumes.

Návaznosti

603437, interní kód MU

Název: SOLUTIONS - Solutions for present and future emerging pollutants in land and water resources management (Akronym: SOLUTIONS)

Investor: Evropská unie, SOLUTIONS - Solutions for present and future emerging pollutants in land and water resources management, Spolupráce

Citovat

SCHULZE, Tobias, Marijan AHEL, Joerg AHLHEIM, Selim AIT-AISSA, Francois BRION, Carolina DI PAOLO, Jean FROMENT, Anita O. HIDASI, Juliane HOLLENDER, Henner HOLLERT, Meng HU, Anett KLOLSS, Sanja KOPRIVICA, Martin KRAUSS, Melis MUZ, Peter OSWALD, Margit PETRE, Jennifer E. SCHOLLEE, Thomas-Benjamin SEILER, Ying SHAO, Jaroslav SLOBODNÍK, Manoj SONAVANE, Marc J. F. SUTER, Knut Erik TOLLEFSEN, Zuzana TOUŠOVÁ, Karl-Heinz WALZ a Werner BRACK. Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis. Science of the Total Environment. Elsevier, 2017, roč. 581, March, s. 350-358. ISSN 0048-9697. Dostupné z: https://dx.doi.org/10.1016/j.scitotenv.2016.12.140.

@article{1410520,
   author = {Schulze, Tobias and Ahel, Marijan and Ahlheim, Joerg and AitandAissa, Selim and Brion, Francois and Di Paolo, Carolina and Froment, Jean and Hidasi, Anita O. and Hollender, Juliane and Hollert, Henner and Hu, Meng and Klolss, Anett and Koprivica, Sanja and Krauss, Martin and Muz, Melis and Oswald, Peter and Petre, Margit and Schollee, Jennifer E. and Seiler, ThomasandBenjamin and Shao, Ying and Slobodník, Jaroslav and Sonavane, Manoj and Suter, Marc J. F. and Tollefsen, Knut Erik and Toušová, Zuzana and Walz, KarlandHeinz and Brack, Werner},
   article_number = {March},
   doi = {http://dx.doi.org/10.1016/j.scitotenv.2016.12.140},
   keywords = {Automated water sampler; Chemical analysis; Bioassay analysis; Effect-based analysis; Applicability domain; Large-volume solid phase extraction; LVSPE},
   language = {eng},
   issn = {0048-9697},
   journal = {Science of the Total Environment},
   title = {Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis},
   url = {https://www.sciencedirect.com/science/article/pii/S0048969716328303?via%3Dihub},
   volume = {581},
   year = {2017}
}

TY  - JOUR
ID  - 1410520
AU  - Schulze, Tobias - Ahel, Marijan - Ahlheim, Joerg - Ait-Aissa, Selim - Brion, Francois - Di Paolo, Carolina - Froment, Jean - Hidasi, Anita O. - Hollender, Juliane - Hollert, Henner - Hu, Meng - Klolss, Anett - Koprivica, Sanja - Krauss, Martin - Muz, Melis - Oswald, Peter - Petre, Margit - Schollee, Jennifer E. - Seiler, Thomas-Benjamin - Shao, Ying - Slobodník, Jaroslav - Sonavane, Manoj - Suter, Marc J. F. - Tollefsen, Knut Erik - Toušová, Zuzana - Walz, Karl-Heinz - Brack, Werner
PY  - 2017
TI  - Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis
JF  - Science of the Total Environment
VL  - 581
IS  - March
SP  - 350-358
EP  - 350-358
PB  - Elsevier
SN  - 00489697
KW  - Automated water sampler
KW  - Chemical analysis
KW  - Bioassay analysis
KW  - Effect-based analysis
KW  - Applicability domain
KW  - Large-volume solid phase extraction
KW  - LVSPE
UR  - https://www.sciencedirect.com/science/article/pii/S0048969716328303?via%3Dihub
L2  - https://www.sciencedirect.com/science/article/pii/S0048969716328303?via%3Dihub
N2  - The implementation of targeted and nontargeted chemical screening analysis in combination with in vitro and organism-level bioassays is a prerequisite for a more holistic monitoring of water quality in the future. For chemical analysis, little or no sample enrichment is often sufficient, while bioanalysis often requires larger sample volumes at a certain enrichment factor for conducting comprehensive bioassays on different endpoints or furthereffect-directed analysis (EDA). To avoid logistic and technical issues related to the storage and transport of large volumes of water, sampling would benefit greatly from onsite extraction. This study presents a novel onsite large volume solid phase extraction (LVSPE) device tailored to fulfill the requirements for the successful effect-based and chemical screening of water resources and complies with available international standards for automated sampling devices. Laboratory recovery experiments using 251 organic compounds in the log D range from -3.6 to 9.4 (at pH 7.0) spiked into pristine water resulted in acceptable recoveries and from 60 to 123% for 159 out of 251 substances. Within a European-wide demonstration program, the LVSPE was able to enrich compounds in concentration ranges over three orders of magnitude (1 ng L-1 to 2400 ng L-1). It was possible to discriminate responsive samples from samples with no or only low effects in a set of six different bioassays "( i.e. acetylcholinesterase and algal growth inhibition, androgenicity, estrogenicity, fish embryo toxicity, glucocorticoid activity). The LVSPE thus proved applicable for onsite extraction of sufficient amounts of water to investigate water quality thoroughly by means of chemical analysis and effect-based tools without the common limitations due to small sample volumes.
ER  -

SCHULZE, Tobias, Marijan AHEL, Joerg AHLHEIM, Selim AIT-AISSA, Francois BRION, Carolina DI PAOLO, Jean FROMENT, Anita O. HIDASI, Juliane HOLLENDER, Henner HOLLERT, Meng HU, Anett KLOLSS, Sanja KOPRIVICA, Martin KRAUSS, Melis MUZ, Peter OSWALD, Margit PETRE, Jennifer E. SCHOLLEE, Thomas-Benjamin SEILER, Ying SHAO, Jaroslav SLOBODNÍK, Manoj SONAVANE, Marc J. F. SUTER, Knut Erik TOLLEFSEN, Zuzana TOUŠOVÁ, Karl-Heinz WALZ a Werner BRACK. Assessment of a novel device for onsite integrative large-volume solid phase extraction of water samples to enable a comprehensive chemical and effect-based analysis. \textit{Science of the Total Environment}. Elsevier, 2017, roč.~581, March, s.~350-358. ISSN~0048-9697. Dostupné z: https://dx.doi.org/10.1016/j.scitotenv.2016.12.140.

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