Characterizing Spatial Diversity of Passive Sampling Sites for
Measuring Levels and Trends of Semivolatile Organic Chemicals

J 2018

Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals

KALINA, Jiří, Martin SCHERINGER, Jana BORŮVKOVÁ, Petr KUKUČKA, Petra PŘIBYLOVÁ et. al.

Základní údaje

Originální název

Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals

Autoři

KALINA, Jiří (203 Česká republika, domácí), Martin SCHERINGER (756 Švýcarsko, domácí), Jana BORŮVKOVÁ (203 Česká republika, domácí), Petr KUKUČKA (203 Česká republika, domácí), Petra PŘIBYLOVÁ (203 Česká republika, domácí), Ondřej SÁŇKA (203 Česká republika, domácí), Lisa Emily MELYMUK (124 Kanada, domácí), Milan VANA (203 Česká republika) a Jana KLÁNOVÁ (203 Česká republika, garant, domácí)

Vydání

ENVIRONMENTAL SCIENCE & TECHNOLOGY, WASHINGTON, AMER CHEMICAL SOC, 2018, 0013-936X

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Spojené státy

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 7.149

Kód RIV

RIV/00216224:14310/18:00104744

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1021/acs.est.8b03414

UT WoS

000445441000041

Klíčová slova anglicky

POLYCYCLIC AROMATIC-HYDROCARBONS; AIR SAMPLERS; POLYCHLORINATED-BIPHENYLS; TEMPORAL TRENDS; AMBIENT AIR; POLLUTANTS; ATMOSPHERE; TOOL; REGION; PAHS

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 1. 12. 2018 21:28, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

Passive air sampling of semivolatile organic compounds (SVOCs) is a relatively inexpensive method that facilitates extensive campaigns with numerous sampling sites. An important question in the design of passive-sampling networks concerns the number and location of samplers. We investigate this question with the example of 17 SVOCs sampled at 14 background sites across the Czech Republic. More than 200 time series (length 5-11 years) were used to characterize SVOC levels and trends in air between 2003 and 2015. Six polychlorinated biphenyls (PCBs), 6 polyaromatic hydrocarbons (PAHs), and 5 organochlorine pesticides (OCPs) at 14 sites were assessed using data from the MONET passive sampling network. Significant decreases were found for most PCBs and OCPs whereas hexachlorobenzene (HCB) and most PAHs showed (mostly insignificant) increases. Spatial variability was rather low for PCBs and OCPs except for dichlorodiphenyltri-chloroethane (DDT) and rather high for PAHs. The variability of the SVOC levels and trends depends on characteristics of the sites including their remoteness, landscape, population, and pollution sources. The sites can be grouped in distinct clusters, which helps to identify similar and, thereby, potentially redundant sites. This information is useful when monitoring networks need to be optimized regarding the location and number of sites.

Návaznosti

CZ.02.1.01/0.0/0.0/16_013/0001315, interní kód MU

Název: ACTRIS - CZ - RI (Akronym: ACTRIS-CZ RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, ACTRIS - CZ - RI, PO 1 Posilování kapacit pro kvalitní výzkum

CZ.02.1.01/0.0/0.0/16_013/0001761, interní kód MU

Název: RECETOX RI - OP VVV (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, RECETOX RI - OP VVV, PO 1 Posilování kapacit pro kvalitní výzkum

EF15_003/0000469, projekt VaV

Název: Cetocoen Plus

LM2015037, projekt VaV

Název: ACTRIS – účast České republiky (Akronym: ACTRIS-CZ)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, ACTRIS-CZ - Aerosol, Clouds and Trace Gases Research Infrastructure Network

LM2015051, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Výzkumná infrastruktura RECETOX

Citovat

KALINA, Jiří, Martin SCHERINGER, Jana BORŮVKOVÁ, Petr KUKUČKA, Petra PŘIBYLOVÁ, Ondřej SÁŇKA, Lisa Emily MELYMUK, Milan VANA a Jana KLÁNOVÁ. Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals. ENVIRONMENTAL SCIENCE & TECHNOLOGY. WASHINGTON: AMER CHEMICAL SOC, 2018, roč. 52, č. 18, s. 10599-10608. ISSN 0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.8b03414.

@article{1473757,
   author = {Kalina, Jiří and Scheringer, Martin and Borůvková, Jana and Kukučka, Petr and Přibylová, Petra and Sáňka, Ondřej and Melymuk, Lisa Emily and Vana, Milan and Klánová, Jana},
   article_location = {WASHINGTON},
   article_number = {18},
   doi = {http://dx.doi.org/10.1021/acs.est.8b03414},
   keywords = {POLYCYCLIC AROMATIC-HYDROCARBONS; AIR SAMPLERS; POLYCHLORINATED-BIPHENYLS; TEMPORAL TRENDS; AMBIENT AIR; POLLUTANTS; ATMOSPHERE; TOOL; REGION; PAHS},
   language = {eng},
   issn = {0013-936X},
   journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY},
   title = {Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals},
   url = {https://pubs.acs.org/doi/10.1021/acs.est.8b03414},
   volume = {52},
   year = {2018}
}

TY  - JOUR
ID  - 1473757
AU  - Kalina, Jiří - Scheringer, Martin - Borůvková, Jana - Kukučka, Petr - Přibylová, Petra - Sáňka, Ondřej - Melymuk, Lisa Emily - Vana, Milan - Klánová, Jana
PY  - 2018
TI  - Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals
JF  - ENVIRONMENTAL SCIENCE & TECHNOLOGY
VL  - 52
IS  - 18
SP  - 10599-10608
EP  - 10599-10608
PB  - AMER CHEMICAL SOC
SN  - 0013936X
KW  - POLYCYCLIC AROMATIC-HYDROCARBONS
KW  - AIR SAMPLERS
KW  - POLYCHLORINATED-BIPHENYLS
KW  - TEMPORAL TRENDS
KW  - AMBIENT AIR
KW  - POLLUTANTS
KW  - ATMOSPHERE
KW  - TOOL
KW  - REGION
KW  - PAHS
UR  - https://pubs.acs.org/doi/10.1021/acs.est.8b03414
L2  - https://pubs.acs.org/doi/10.1021/acs.est.8b03414
N2  - Passive air sampling of semivolatile organic compounds (SVOCs) is a relatively inexpensive method that facilitates extensive campaigns with numerous sampling sites. An important question in the design of passive-sampling networks concerns the number and location of samplers. We investigate this question with the example of 17 SVOCs sampled at 14 background sites across the Czech Republic. More than 200 time series (length 5-11 years) were used to characterize SVOC levels and trends in air between 2003 and 2015. Six polychlorinated biphenyls (PCBs), 6 polyaromatic hydrocarbons (PAHs), and 5 organochlorine pesticides (OCPs) at 14 sites were assessed using data from the MONET passive sampling network. Significant decreases were found for most PCBs and OCPs whereas hexachlorobenzene (HCB) and most PAHs showed (mostly insignificant) increases. Spatial variability was rather low for PCBs and OCPs except for dichlorodiphenyltri-chloroethane (DDT) and rather high for PAHs. The variability of the SVOC levels and trends depends on characteristics of the sites including their remoteness, landscape, population, and pollution sources. The sites can be grouped in distinct clusters, which helps to identify similar and, thereby, potentially redundant sites. This information is useful when monitoring networks need to be optimized regarding the location and number of sites.
ER  -

KALINA, Jiří, Martin SCHERINGER, Jana BORŮVKOVÁ, Petr KUKUČKA, Petra PŘIBYLOVÁ, Ondřej SÁŇKA, Lisa Emily MELYMUK, Milan VANA a Jana KLÁNOVÁ. Characterizing Spatial Diversity of Passive Sampling Sites for Measuring Levels and Trends of Semivolatile Organic Chemicals. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2018, roč.~52, č.~18, s.~10599-10608. ISSN~0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.8b03414.

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