Linking past uses of legacy SVOCs with today's indoor levels
and human exposure

J 2019

Linking past uses of legacy SVOCs with today's indoor levels and human exposure

DEMIRTEPE, Hale, Lisa Emily MELYMUK, Miriam Leah DIAMOND, Lola Murielle BAJARD ÉP.ESNER, Šimon VOJTA et. al.

Základní údaje

Originální název

Linking past uses of legacy SVOCs with today's indoor levels and human exposure

Autoři

DEMIRTEPE, Hale (792 Turecko, domácí), Lisa Emily MELYMUK (124 Kanada, domácí), Miriam Leah DIAMOND (124 Kanada), Lola Murielle BAJARD ÉP.ESNER (250 Francie, domácí), Šimon VOJTA (203 Česká republika, domácí), Roman PROKEŠ (203 Česká republika, domácí), Ondřej SÁŇKA (203 Česká republika, domácí), Jana KLÁNOVÁ (203 Česká republika, garant, domácí), L'ubica MURÍNOVÁ (703 Slovensko), Denisa RICHTEROVA (703 Slovensko), Vladimira RASPLOVA (703 Slovensko) a Tomáš TRNOVEC (703 Slovensko)

Vydání

Environment International, OXFORD, PERGAMON-ELSEVIER SCIENCE LTD, 2019, 0160-4120

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Velká Británie a Severní Irsko

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 7.577

Kód RIV

RIV/00216224:14310/19:00110322

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1016/j.envint.2019.04.001

UT WoS

000467383500064

Klíčová slova anglicky

Human intake; Indoor environment; Flame retardants; Legacy POPs; PAHs; Risk prioritization

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 23. 3. 2020 16:52, Mgr. Marie Šípková, DiS.

Anotace

V originále

Semivolatile organic compounds (SVOCs) emitted from consumer products, building materials, and indoor and outdoor activities can be highly persistent in indoor environments. Human exposure to and environmental contamination with polychlorinated biphenyls (PCBs) was previously reported in a region near a former PCB production facility in Slovakia. However, we found that the indoor residential PCB levels did not correlate with the distance from the facility. Rather, indoor levels in this region and those reported in the literature were related to the historic PCB use on a national scale and the inferred presence of primary sources of PCBs in the homes. Other SVOCs had levels linked with either the activities in the home, e.g., polycyclic aromatic hydrocarbons (PAHs) with wood heating; or outdoor activities, e.g., organochlorine pesticides (OCPs) with agricultural land use and building age. We propose a classification framework to prioritize SVOCs for monitoring in indoor environments and to evaluate risks from indoor SVOC exposures. Application of this framework to 88 measured SVOCs identified several PCB congeners (CB-11, -28, -52), hexachlorobenzene (HCB), benzo(a)pyrene, and gamma-HCH as priority compounds based on high exposure and toxicity assessed by means of toxicity reference values (TRVs). Application of the framework to many emerging compounds such as novel flame retardants was not possible because of either no or outdated TRVs. Concurrent identification of seven SVOC groups in indoor environments provided information on their comparative levels and distributions, their sources, and informed our assessment of associated risks.

Návaznosti

EF16_013/0001761, projekt VaV

Název: RECETOX RI

LM2015051, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Výzkumná infrastruktura RECETOX

LO1214, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Centrum pro výzkum toxických látek v prostředí

733032, interní kód MU

Název: European Human Biomonitoring Initiative (Akronym: HBM4EU)

Investor: Evropská unie, European Human Biomonitoring Initiative, Health, demographic change and wellbeing (Societal Challenges)

734522, interní kód MU

Název: Synergising International Research Studies into the Environmental Fate and Behaviour of Toxic Organic Chemicals in the Waste Stream (Akronym: INTERWASTE)

Investor: Evropská unie, Synergising International Research Studies into the Environmental Fate and Behaviour of Toxic Organic Chemicals in the Waste Stream, MSCA Marie Skłodowska-Curie Actions (Excellent Science)

Citovat

DEMIRTEPE, Hale, Lisa Emily MELYMUK, Miriam Leah DIAMOND, Lola Murielle BAJARD ÉP.ESNER, Šimon VOJTA, Roman PROKEŠ, Ondřej SÁŇKA, Jana KLÁNOVÁ, L'ubica MURÍNOVÁ, Denisa RICHTEROVA, Vladimira RASPLOVA a Tomáš TRNOVEC. Linking past uses of legacy SVOCs with today's indoor levels and human exposure. Environment International. OXFORD: PERGAMON-ELSEVIER SCIENCE LTD, 2019, roč. 127, June, s. 653-663. ISSN 0160-4120. Dostupné z: https://dx.doi.org/10.1016/j.envint.2019.04.001.

@article{1548600,
   author = {Demirtepe, Hale and Melymuk, Lisa Emily and Diamond, Miriam Leah and Bajard ép.Esner, Lola Murielle and Vojta, Šimon and Prokeš, Roman and Sáňka, Ondřej and Klánová, Jana and Murínová, L'ubica and Richterova, Denisa and Rasplova, Vladimira and Trnovec, Tomáš},
   article_location = {OXFORD},
   article_number = {June},
   doi = {http://dx.doi.org/10.1016/j.envint.2019.04.001},
   keywords = {Human intake; Indoor environment; Flame retardants; Legacy POPs; PAHs; Risk prioritization},
   language = {eng},
   issn = {0160-4120},
   journal = {Environment International},
   title = {Linking past uses of legacy SVOCs with today's indoor levels and human exposure},
   url = {https://www.sciencedirect.com/science/article/pii/S0160412018327119?via%3Dihub},
   volume = {127},
   year = {2019}
}

TY  - JOUR
ID  - 1548600
AU  - Demirtepe, Hale - Melymuk, Lisa Emily - Diamond, Miriam Leah - Bajard ép.Esner, Lola Murielle - Vojta, Šimon - Prokeš, Roman - Sáňka, Ondřej - Klánová, Jana - Murínová, L'ubica - Richterova, Denisa - Rasplova, Vladimira - Trnovec, Tomáš
PY  - 2019
TI  - Linking past uses of legacy SVOCs with today's indoor levels and human exposure
JF  - Environment International
VL  - 127
IS  - June
SP  - 653-663
EP  - 653-663
PB  - PERGAMON-ELSEVIER SCIENCE LTD
SN  - 01604120
KW  - Human intake
KW  - Indoor environment
KW  - Flame retardants
KW  - Legacy POPs
KW  - PAHs
KW  - Risk prioritization
UR  - https://www.sciencedirect.com/science/article/pii/S0160412018327119?via%3Dihub
L2  - https://www.sciencedirect.com/science/article/pii/S0160412018327119?via%3Dihub
N2  - Semivolatile organic compounds (SVOCs) emitted from consumer products, building materials, and indoor and outdoor activities can be highly persistent in indoor environments. Human exposure to and environmental contamination with polychlorinated biphenyls (PCBs) was previously reported in a region near a former PCB production facility in Slovakia. However, we found that the indoor residential PCB levels did not correlate with the distance from the facility. Rather, indoor levels in this region and those reported in the literature were related to the historic PCB use on a national scale and the inferred presence of primary sources of PCBs in the homes. Other SVOCs had levels linked with either the activities in the home, e.g., polycyclic aromatic hydrocarbons (PAHs) with wood heating; or outdoor activities, e.g., organochlorine pesticides (OCPs) with agricultural land use and building age. We propose a classification framework to prioritize SVOCs for monitoring in indoor environments and to evaluate risks from indoor SVOC exposures. Application of this framework to 88 measured SVOCs identified several PCB congeners (CB-11, -28, -52), hexachlorobenzene (HCB), benzo(a)pyrene, and gamma-HCH as priority compounds based on high exposure and toxicity assessed by means of toxicity reference values (TRVs). Application of the framework to many emerging compounds such as novel flame retardants was not possible because of either no or outdated TRVs. Concurrent identification of seven SVOC groups in indoor environments provided information on their comparative levels and distributions, their sources, and informed our assessment of associated risks.
ER  -

DEMIRTEPE, Hale, Lisa Emily MELYMUK, Miriam Leah DIAMOND, Lola Murielle BAJARD ÉP.ESNER, Šimon VOJTA, Roman PROKEŠ, Ondřej SÁŇKA, Jana KLÁNOVÁ, L'ubica MURÍNOVÁ, Denisa RICHTEROVA, Vladimira RASPLOVA a Tomáš TRNOVEC. Linking past uses of legacy SVOCs with today's indoor levels and human exposure. \textit{Environment International}. OXFORD: PERGAMON-ELSEVIER SCIENCE LTD, 2019, roč.~127, June, s.~653-663. ISSN~0160-4120. Dostupné z: https://dx.doi.org/10.1016/j.envint.2019.04.001.

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