Bulk atmospheric deposition of persistent organic pollutants
and polycyclic aromatic hydrocarbons in Central Europe

J 2019

Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe

NEŽIKOVÁ, Barbora, Céline DEGRENDELE, Pavel ČUPR, P. HOHENBLUM, W. MOCHE et. al.

Základní údaje

Originální název

Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe

Autoři

NEŽIKOVÁ, Barbora (203 Česká republika, domácí), Céline DEGRENDELE (250 Francie, domácí), Pavel ČUPR (203 Česká republika, domácí), P. HOHENBLUM, W. MOCHE, Roman PROKEŠ (203 Česká republika, domácí), Lenka VAŇKOVÁ (203 Česká republika, domácí), Petr KUKUČKA (203 Česká republika, domácí), Jakub MARTINÍK (203 Česká republika, domácí), Ondřej AUDY (203 Česká republika, domácí), Petra PŘIBYLOVÁ (203 Česká republika, domácí), Ivan HOLOUBEK (203 Česká republika, domácí), P. WEISS, Jana KLÁNOVÁ (203 Česká republika, domácí) a Gerhard LAMMEL (276 Německo, garant, domácí)

Vydání

Environmental Science and Pollution Research, Heidelberg, Springer Heidelberg, 2019, 0944-1344

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Německo

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 3.056

Kód RIV

RIV/00216224:14310/19:00108200

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1007/s11356-019-05464-9

UT WoS

000477958300020

Klíčová slova anglicky

Bulk atmospheric deposition; POPs; PCBs; OCPs; PAHs; Central Europe; Deposition fluxes

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 3. 4. 2020 12:54, Mgr. Marie Šípková, DiS.

Anotace

V originále

Polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) are ubiquitous and toxic contaminants. Their atmospheric deposition fluxes on the regional scale were quantified based on simultaneous sampling during 1 to 5 years at 1 to 6 background/rural sites in the Czech Republic and Austria. The samples were extracted and analysed by means of gas chromatography coupled to mass spectrometry. For all seasons and sites, total deposition fluxes for Sigma(15)PAHs ranged 23-1100 ng m(-2) d(-1), while those for Sigma 6PCBs and Sigma 12OCPs ranged 64-4400 and 410-7800 pg m(-2) d(-1), respectively. Fluoranthene and pyrene were the main contributors to the PAH deposition fluxes, accounting on average for 19% each, while deposition fluxes of PCBs and OCPs were dominated by PCB153 (26%) and gamma-hexachlorobenzene (30%), respectively. The highest deposition flux of Sigma(15)PAHs was generally found in spring, while no seasonality was found for PCB deposition. For deposition fluxes for Sigma(12)OCPs, no clear spatial trend was found, confirming the perception of long-lived regional pollutants. Although most OCPs and PCBs hardly partition to the particulate phase in ambient air, on average, 42% of their deposition fluxes were found on filters, confirming the perception that particle deposition is more efficient than dry gaseous deposition. Due to methodological constraints, fluxes derived from bulk deposition samplers should be understood as lower estimates, in particular with regard to those substances which in ambient aerosols mostly partition to the particulate phase.

Návaznosti

GA16-11537S, projekt VaV

Název: Transformační produkty mono- a polyaromatických uhlovodíků v atmosferických aerosolech – prioritní nebezpečné polutanty

Investor: Grantová agentura ČR, Transformační produkty mono- a polyaromatických uhlovodíků v atmosferických aerosolech – prioritní nebezpečné polutanty

LM2015037, projekt VaV

Název: ACTRIS – účast České republiky (Akronym: ACTRIS-CZ)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, ACTRIS-CZ - Aerosol, Clouds and Trace Gases Research Infrastructure Network

LM2015051, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Výzkumná infrastruktura RECETOX

M00124, interní kód MU

Název: MONAIRNET (Akronym: MONAIRNET)

Investor: Úřad spolkové vlády Dolního Rakouska, MONAIRNET, 2. Regionální dostupnost a udržitelný rozvoj

Citovat

NEŽIKOVÁ, Barbora, Céline DEGRENDELE, Pavel ČUPR, P. HOHENBLUM, W. MOCHE, Roman PROKEŠ, Lenka VAŇKOVÁ, Petr KUKUČKA, Jakub MARTINÍK, Ondřej AUDY, Petra PŘIBYLOVÁ, Ivan HOLOUBEK, P. WEISS, Jana KLÁNOVÁ a Gerhard LAMMEL. Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe. Environmental Science and Pollution Research. Heidelberg: Springer Heidelberg, 2019, roč. 26, č. 23, s. 23429-23441. ISSN 0944-1344. Dostupné z: https://dx.doi.org/10.1007/s11356-019-05464-9.

@article{1639340,
   author = {Nežiková, Barbora and Degrendele, Céline and Čupr, Pavel and Hohenblum, P. and Moche, W. and Prokeš, Roman and Vaňková, Lenka and Kukučka, Petr and Martiník, Jakub and Audy, Ondřej and Přibylová, Petra and Holoubek, Ivan and Weiss, P. and Klánová, Jana and Lammel, Gerhard},
   article_location = {Heidelberg},
   article_number = {23},
   doi = {http://dx.doi.org/10.1007/s11356-019-05464-9},
   keywords = {Bulk atmospheric deposition; POPs; PCBs; OCPs; PAHs; Central Europe; Deposition fluxes},
   language = {eng},
   issn = {0944-1344},
   journal = {Environmental Science and Pollution Research},
   title = {Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe},
   url = {http://dx.doi.org/10.1007/s11356-019-05464-9},
   volume = {26},
   year = {2019}
}

TY  - JOUR
ID  - 1639340
AU  - Nežiková, Barbora - Degrendele, Céline - Čupr, Pavel - Hohenblum, P. - Moche, W. - Prokeš, Roman - Vaňková, Lenka - Kukučka, Petr - Martiník, Jakub - Audy, Ondřej - Přibylová, Petra - Holoubek, Ivan - Weiss, P. - Klánová, Jana - Lammel, Gerhard
PY  - 2019
TI  - Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe
JF  - Environmental Science and Pollution Research
VL  - 26
IS  - 23
SP  - 23429-23441
EP  - 23429-23441
PB  - Springer Heidelberg
SN  - 09441344
KW  - Bulk atmospheric deposition
KW  - POPs
KW  - PCBs
KW  - OCPs
KW  - PAHs
KW  - Central Europe
KW  - Deposition fluxes
UR  - http://dx.doi.org/10.1007/s11356-019-05464-9
L2  - http://dx.doi.org/10.1007/s11356-019-05464-9
N2  - Polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) are ubiquitous and toxic contaminants. Their atmospheric deposition fluxes on the regional scale were quantified based on simultaneous sampling during 1 to 5 years at 1 to 6 background/rural sites in the Czech Republic and Austria. The samples were extracted and analysed by means of gas chromatography coupled to mass spectrometry. For all seasons and sites, total deposition fluxes for Sigma(15)PAHs ranged 23-1100 ng m(-2) d(-1), while those for Sigma 6PCBs and Sigma 12OCPs ranged 64-4400 and 410-7800 pg m(-2) d(-1), respectively. Fluoranthene and pyrene were the main contributors to the PAH deposition fluxes, accounting on average for 19% each, while deposition fluxes of PCBs and OCPs were dominated by PCB153 (26%) and gamma-hexachlorobenzene (30%), respectively. The highest deposition flux of Sigma(15)PAHs was generally found in spring, while no seasonality was found for PCB deposition. For deposition fluxes for Sigma(12)OCPs, no clear spatial trend was found, confirming the perception of long-lived regional pollutants. Although most OCPs and PCBs hardly partition to the particulate phase in ambient air, on average, 42% of their deposition fluxes were found on filters, confirming the perception that particle deposition is more efficient than dry gaseous deposition. Due to methodological constraints, fluxes derived from bulk deposition samplers should be understood as lower estimates, in particular with regard to those substances which in ambient aerosols mostly partition to the particulate phase.
ER  -

NEŽIKOVÁ, Barbora, Céline DEGRENDELE, Pavel ČUPR, P. HOHENBLUM, W. MOCHE, Roman PROKEŠ, Lenka VAŇKOVÁ, Petr KUKUČKA, Jakub MARTINÍK, Ondřej AUDY, Petra PŘIBYLOVÁ, Ivan HOLOUBEK, P. WEISS, Jana KLÁNOVÁ a Gerhard LAMMEL. Bulk atmospheric deposition of persistent organic pollutants and polycyclic aromatic hydrocarbons in Central Europe. \textit{Environmental Science and Pollution Research}. Heidelberg: Springer Heidelberg, 2019, roč.~26, č.~23, s.~23429-23441. ISSN~0944-1344. Dostupné z: https://dx.doi.org/10.1007/s11356-019-05464-9.

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