Comparability of long-term temporal trends of POPs from
co-located active and passive air monitoring networks in Europe

J 2019

Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe

KALINA, Jiří, Kevin Bradley WHITE, Martin SCHERINGER, Petra PŘIBYLOVÁ, Petr KUKUČKA et. al.

Základní údaje

Originální název

Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe

Autoři

KALINA, Jiří (203 Česká republika, domácí), Kevin Bradley WHITE (124 Kanada, domácí), Martin SCHERINGER (756 Švýcarsko, domácí), Petra PŘIBYLOVÁ (203 Česká republika, domácí), Petr KUKUČKA (203 Česká republika, domácí), Ondřej AUDY (203 Česká republika, domácí) a Jana KLÁNOVÁ (203 Česká republika, garant, domácí)

Vydání

ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS, CAMBRIDGE, ROYAL SOC CHEMISTRY, 2019, 2050-7887

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10406 Analytical chemistry

Stát vydavatele

Velká Británie a Severní Irsko

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 3.238

Kód RIV

RIV/00216224:14310/19:00113359

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1039/c9em00136k

UT WoS

000475800200004

Klíčová slova anglicky

PERSISTENT ORGANIC POLLUTANTS; POLYCHLORINATED-BIPHENYLS; POTENTIAL SOURCES; SEASONAL TRENDS; AMBIENT AIR; SAMPLERS; PCBS; ATMOSPHERE; CALIBRATION; PBDES

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 3. 4. 2020 13:31, Mgr. Marie Šípková, DiS.

Anotace

V originále

The comparability of data from active (ACT) and passive sampling (PAS) of persistent organic pollutants (POPs) in air is hindered by uncertainties related to the derivation of sampling rates and concentrations, as well as differences in the duration, volume and frequency of sampling. Although data from ACT have been used extensively in short-term PAS calibration studies, no attempts have been made to evaluate the comparability of long-term trends calculated from PAS to established ACT trends. This is crucial, as continuous long-term ACT is unfeasible in most regions of the world. To address these challenges, we calculated and compared trends for organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs) and polybrominated diphenyl ethers (PBDEs) at the six sites in Europe with at least 5 years of co-located ACT and PAS data (2012-2016): Birkenes, Kosetice, Pallas, Rao, Storhofoi and Zeppelin. Strong agreement of ACT and PAS trends was observed for most OCPs and PCBs. Apart from two PCBs at Storhofoi, all pairs of ACT and PAS trends followed the same direction. However, differences in the magnitude, significance and confidence intervals of their slopes were observed for some compounds and were primarily attributed to the short duration of the PAS time series. Despite some limitations, our results suggest that the comparability of ACT and PAS POP trends will continue to improve with additional years of data. This study confirms the suitability of PAS for the calculation of long-term POP trends in air, and highlights the importance of continuous sampling at established monitoring sites with consistent analytical methods.

Návaznosti

EF15_003/0000469, projekt VaV

Název: Cetocoen Plus

EF16_013/0001761, projekt VaV

Název: RECETOX RI

LM2015037, projekt VaV

Název: ACTRIS – účast České republiky (Akronym: ACTRIS-CZ)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, ACTRIS-CZ - Aerosol, Clouds and Trace Gases Research Infrastructure Network

LM2015051, projekt VaV

Název: Centrum pro výzkum toxických látek v prostředí (Akronym: RECETOX RI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Výzkumná infrastruktura RECETOX

689443, interní kód MU

Název: ERA-PLANET - The European network for observing our changing planet (Akronym: ERA-PLANET)

Investor: Evropská unie, ERA-PLANET - The European network for observing our changing planet, Climate action, environment, resource efficiency and raw materials (Societal Challenges)

Citovat

KALINA, Jiří, Kevin Bradley WHITE, Martin SCHERINGER, Petra PŘIBYLOVÁ, Petr KUKUČKA, Ondřej AUDY a Jana KLÁNOVÁ. Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe. ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS. CAMBRIDGE: ROYAL SOC CHEMISTRY, 2019, roč. 21, č. 7, s. 1132-1142. ISSN 2050-7887. Dostupné z: https://dx.doi.org/10.1039/c9em00136k.

@article{1639542,
   author = {Kalina, Jiří and White, Kevin Bradley and Scheringer, Martin and Přibylová, Petra and Kukučka, Petr and Audy, Ondřej and Klánová, Jana},
   article_location = {CAMBRIDGE},
   article_number = {7},
   doi = {http://dx.doi.org/10.1039/c9em00136k},
   keywords = {PERSISTENT ORGANIC POLLUTANTS; POLYCHLORINATED-BIPHENYLS; POTENTIAL SOURCES; SEASONAL TRENDS; AMBIENT AIR; SAMPLERS; PCBS; ATMOSPHERE; CALIBRATION; PBDES},
   language = {eng},
   issn = {2050-7887},
   journal = {ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS},
   title = {Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe},
   url = {http://dx.doi.org/10.1039/c9em00136k},
   volume = {21},
   year = {2019}
}

TY  - JOUR
ID  - 1639542
AU  - Kalina, Jiří - White, Kevin Bradley - Scheringer, Martin - Přibylová, Petra - Kukučka, Petr - Audy, Ondřej - Klánová, Jana
PY  - 2019
TI  - Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe
JF  - ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS
VL  - 21
IS  - 7
SP  - 1132-1142
EP  - 1132-1142
PB  - ROYAL SOC CHEMISTRY
SN  - 20507887
KW  - PERSISTENT ORGANIC POLLUTANTS
KW  - POLYCHLORINATED-BIPHENYLS
KW  - POTENTIAL SOURCES
KW  - SEASONAL TRENDS
KW  - AMBIENT AIR
KW  - SAMPLERS
KW  - PCBS
KW  - ATMOSPHERE
KW  - CALIBRATION
KW  - PBDES
UR  - http://dx.doi.org/10.1039/c9em00136k
L2  - http://dx.doi.org/10.1039/c9em00136k
N2  - The comparability of data from active (ACT) and passive sampling (PAS) of persistent organic pollutants (POPs) in air is hindered by uncertainties related to the derivation of sampling rates and concentrations, as well as differences in the duration, volume and frequency of sampling. Although data from ACT have been used extensively in short-term PAS calibration studies, no attempts have been made to evaluate the comparability of long-term trends calculated from PAS to established ACT trends. This is crucial, as continuous long-term ACT is unfeasible in most regions of the world. To address these challenges, we calculated and compared trends for organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs) and polybrominated diphenyl ethers (PBDEs) at the six sites in Europe with at least 5 years of co-located ACT and PAS data (2012-2016): Birkenes, Kosetice, Pallas, Rao, Storhofoi and Zeppelin. Strong agreement of ACT and PAS trends was observed for most OCPs and PCBs. Apart from two PCBs at Storhofoi, all pairs of ACT and PAS trends followed the same direction. However, differences in the magnitude, significance and confidence intervals of their slopes were observed for some compounds and were primarily attributed to the short duration of the PAS time series. Despite some limitations, our results suggest that the comparability of ACT and PAS POP trends will continue to improve with additional years of data. This study confirms the suitability of PAS for the calculation of long-term POP trends in air, and highlights the importance of continuous sampling at established monitoring sites with consistent analytical methods.
ER  -

KALINA, Jiří, Kevin Bradley WHITE, Martin SCHERINGER, Petra PŘIBYLOVÁ, Petr KUKUČKA, Ondřej AUDY a Jana KLÁNOVÁ. Comparability of long-term temporal trends of POPs from co-located active and passive air monitoring networks in Europe. \textit{ENVIRONMENTAL SCIENCE-PROCESSES \&{}amp; IMPACTS}. CAMBRIDGE: ROYAL SOC CHEMISTRY, 2019, roč.~21, č.~7, s.~1132-1142. ISSN~2050-7887. Dostupné z: https://dx.doi.org/10.1039/c9em00136k.

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