KOŠŤÁL, Michal, Martin SCHULC, Losa EVŽEN, Zdeněk MATĚJ, František CVACHOVEC, Filip MRAVEC, Filip BRIJAR, Tomáš CZAKOJ, Jan ŠIMON, Šimon VADJÁK, Michal ANTOŠ, Václav PŘENOSIL, Vojtěch RYPAR, Marek ZMEŠKAL and Roberto CAPOTE. Characterization of the neutron flux on the surface of a liquid water target intended for 18F production. Radiation Physics and Chemistry. Elsevier, 2021, vol. 184, No 109475, p. 1-13. ISSN 0969-806X. Available from: https://dx.doi.org/10.1016/j.radphyschem.2021.109475.
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Basic information
Original name Characterization of the neutron flux on the surface of a liquid water target intended for 18F production
Authors KOŠŤÁL, Michal (203 Czech Republic, guarantor), Martin SCHULC (203 Czech Republic), Losa EVŽEN (203 Czech Republic), Zdeněk MATĚJ (203 Czech Republic, belonging to the institution), František CVACHOVEC (203 Czech Republic), Filip MRAVEC (203 Czech Republic, belonging to the institution), Filip BRIJAR (203 Czech Republic), Tomáš CZAKOJ (203 Czech Republic), Jan ŠIMON (203 Czech Republic), Šimon VADJÁK (203 Czech Republic), Michal ANTOŠ (203 Czech Republic), Václav PŘENOSIL (203 Czech Republic, belonging to the institution), Vojtěch RYPAR (203 Czech Republic), Marek ZMEŠKAL and Roberto CAPOTE.
Edition Radiation Physics and Chemistry, Elsevier, 2021, 0969-806X.
Other information
Original language English
Type of outcome Article in a journal
Field of Study 10304 Nuclear physics
Country of publisher United Kingdom of Great Britain and Northern Ireland
Confidentiality degree is not subject to a state or trade secret
WWW URL
Impact factor Impact factor: 2.776
RIV identification code RIV/00216224:14330/21:00120061
Organization unit Faculty of Informatics
Doi http://dx.doi.org/10.1016/j.radphyschem.2021.109475
UT WoS 000655297900005
Keywords in English PET;IBA;XXL target;Neutron spectrometry;Cyclotron;Radiation protection
Changed by Changed by: RNDr. Pavel Šmerk, Ph.D., učo 3880. Changed: 28/4/2022 10:08.
Abstract
8F is an important radioisotope used in nuclear medicine for diagnostic purposes. It is produced most often via 18O (p,n)18F reaction. During its production, the oxygen contained in the H218O molecules placed in the cooled target is irradiated by accelerated protons. The production of each 18F atom is accompanied by anisotropic highenergy neutron emission, which is a problem for ensuring radiation safety. These neutrons are responsible for the high radiation dose in a cyclotron pit during 18F production as well as for activation of cyclotron components or might be responsible even for target material changes due to their high penetration properties. A precise characterization of a neutron field on the surface of the liquid water target, used for 18F production, is presented. The neutron flux characterization is performed both by using large-area activation detectors and stilbene detectors at 1 m from the target in a forward direction. The experiments show significant discrepancies between calculated and measured reaction rates in higher threshold reactions 58Ni(n,x)57Co and 51V (n,alpha)48Sc, confirming that the current neutron production reaction models are not suitable for the characterization of the secondary neutrons leaking from the target.
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VI20192022116, research and development projectName: Metody přenosu a detekce scintilačního záření s optickými vlákny a energetickým rozlišením zdrojů ionizujícího záření (Acronym: SIREM)
Investor: Ministry of the Interior of the CR
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