Passive-Sampler-Derived PCB and OCP Concentrations in the
Waters of the World─First Results from the AQUA-GAPS/MONET
Network

J 2023

Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network

LOHMANN, Rainer, Branislav VRANA, Derek MUIR, Foppe SMEDES, Jaromír SOBOTKA et. al.

Základní údaje

Originální název

Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network

Autoři

LOHMANN, Rainer, Branislav VRANA (703 Slovensko, domácí), Derek MUIR, Foppe SMEDES (528 Nizozemské království, domácí), Jaromír SOBOTKA (203 Česká republika, domácí), Eddy Y. ZENG, Lian-Jun BAO, Ian J. ALLAN, Peleg ASTRAHAN, Ricardo O. BARRA, Terry BIDLEMAN, Evgen DYKYI, Nicolas ESTOPPEY, Gilberto FILLMANN (76 Brazílie), Naomi GREENWOOD, Paul A. HELM, Liisa JANTUNEN, Sarit KASERZON, J. Vinicio MACIAS, Keith A. MARUYA, Francisco MOLINA, Brent NEWMAN, Raimon M. PRATS, Manolis TSAPAKIS, Mats TYSKLIND, Barend L. VAN DROOGE, Cameron J. VEAL a Charles S. WONG

Vydání

Environmental Science and Technology, American Chemical Society, 2023, 0013-936X

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Spojené státy

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 11.400 v roce 2022

Kód RIV

RIV/00216224:14310/23:00131417

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1021/acs.est.3c01866

UT WoS

001006294300001

Klíčová slova anglicky

passive sampler; polychlorinated biphenyls; hexachlorobenzene; hexachlorocyclohexanes; organochlorinepesticides; cyclodiene pesticides; global fractionation; silicone rubber; long-range transport

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 18. 4. 2024 10:17, Mgr. Marie Šípková, DiS.

Anotace

V originále

Persistent organic pollutants (POPs) are recognized aspollutantsof global concern, but so far, information on the trends of legacyPOPs in the waters of the world has been missing due to logistical,analytical, and financial reasons. Passive samplers have emerged asan attractive alternative to active water sampling methods as theyaccumulate POPs, represent time-weighted average concentrations, andcan easily be shipped and deployed. As part of the AQUA-GAPS/MONET,passive samplers were deployed at 40 globally distributed sites between2016 and 2020, for a total of 21 freshwater and 40 marine deployments.Results from silicone passive samplers showed & alpha;-hexachlorocyclohexane(HCH) and & gamma;-HCH displaying the greatest concentrations in thenorthern latitudes/Arctic Ocean, in stark contrast to the more persistentpenta (PeCB)- and hexachlorobenzene (HCB), which approached equilibriumacross sampling sites. Geospatial patterns of polychlorinated biphenyl(PCB) aqueous concentrations closely matched original estimates ofproduction and use, implying limited global transport. Positive correlationsbetween log-transformed concentrations of & sigma;7PCB,& sigma;DDTs, & sigma;endosulfan, and & sigma;chlordane, but not & sigma;HCH,and the log of population density (p < 0.05) within5 and 10 km of the sampling sites also supported limited transportfrom used sites. These results help to understand the extent of globaldistribution, and eventually time-trends, of organic pollutants inaquatic systems, such as across freshwaters and oceans. Future deploymentswill aim to establish time-trends at selected sites while adding tothe geographical coverage.

Návaznosti

EF17_043/0009632, projekt VaV

Název: CETOCOEN Excellence

GX20-04676X, projekt VaV

Název: Holistická charakterizace expozice a potenciálních účinků komplexních směsí chemických látek ve vodním prostředí

Investor: Grantová agentura ČR, Holistická charakterizace expozice a potenciálních účinků komplexních směsí chemických látek ve vodním prostředí

857560, interní kód MU
(Kód CEP: EF17_043/0009632)

Název: CETOCOEN Excellence (Akronym: CETOCOEN Excellence)

Investor: Evropská unie, CETOCOEN Excellence, Spreading excellence and widening participation

90121, velká výzkumná infrastruktura

Název: RECETOX RI

Citovat

LOHMANN, Rainer, Branislav VRANA, Derek MUIR, Foppe SMEDES, Jaromír SOBOTKA, Eddy Y. ZENG, Lian-Jun BAO, Ian J. ALLAN, Peleg ASTRAHAN, Ricardo O. BARRA, Terry BIDLEMAN, Evgen DYKYI, Nicolas ESTOPPEY, Gilberto FILLMANN, Naomi GREENWOOD, Paul A. HELM, Liisa JANTUNEN, Sarit KASERZON, J. Vinicio MACIAS, Keith A. MARUYA, Francisco MOLINA, Brent NEWMAN, Raimon M. PRATS, Manolis TSAPAKIS, Mats TYSKLIND, Barend L. VAN DROOGE, Cameron J. VEAL a Charles S. WONG. Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network. Environmental Science and Technology. American Chemical Society, 2023, roč. 57, č. 25, s. 9342-9352. ISSN 0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.3c01866.

@article{2302499,
   author = {Lohmann, Rainer and Vrana, Branislav and Muir, Derek and Smedes, Foppe and Sobotka, Jaromír and Zeng, Eddy Y. and Bao, LianandJun and Allan, Ian J. and Astrahan, Peleg and Barra, Ricardo O. and Bidleman, Terry and Dykyi, Evgen and Estoppey, Nicolas and Fillmann, Gilberto and Greenwood, Naomi and Helm, Paul A. and Jantunen, Liisa and Kaserzon, Sarit and Macias, J. Vinicio and Maruya, Keith A. and Molina, Francisco and Newman, Brent and Prats, Raimon M. and Tsapakis, Manolis and Tysklind, Mats and van Drooge, Barend L. and Veal, Cameron J. and Wong, Charles S.},
   article_number = {25},
   doi = {http://dx.doi.org/10.1021/acs.est.3c01866},
   keywords = {passive sampler; polychlorinated biphenyls; hexachlorobenzene; hexachlorocyclohexanes; organochlorinepesticides; cyclodiene pesticides; global fractionation; silicone rubber; long-range transport},
   language = {eng},
   issn = {0013-936X},
   journal = {Environmental Science and Technology},
   title = {Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network},
   url = {https://pubs.acs.org/doi/10.1021/acs.est.3c01866},
   volume = {57},
   year = {2023}
}

TY  - JOUR
ID  - 2302499
AU  - Lohmann, Rainer - Vrana, Branislav - Muir, Derek - Smedes, Foppe - Sobotka, Jaromír - Zeng, Eddy Y. - Bao, Lian-Jun - Allan, Ian J. - Astrahan, Peleg - Barra, Ricardo O. - Bidleman, Terry - Dykyi, Evgen - Estoppey, Nicolas - Fillmann, Gilberto - Greenwood, Naomi - Helm, Paul A. - Jantunen, Liisa - Kaserzon, Sarit - Macias, J. Vinicio - Maruya, Keith A. - Molina, Francisco - Newman, Brent - Prats, Raimon M. - Tsapakis, Manolis - Tysklind, Mats - van Drooge, Barend L. - Veal, Cameron J. - Wong, Charles S.
PY  - 2023
TI  - Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network
JF  - Environmental Science and Technology
VL  - 57
IS  - 25
SP  - 9342-9352
EP  - 9342-9352
PB  - American Chemical Society
SN  - 0013936X
KW  - passive sampler
KW  - polychlorinated biphenyls
KW  - hexachlorobenzene
KW  - hexachlorocyclohexanes
KW  - organochlorinepesticides
KW  - cyclodiene pesticides
KW  - global fractionation
KW  - silicone rubber
KW  - long-range transport
UR  - https://pubs.acs.org/doi/10.1021/acs.est.3c01866
N2  - Persistent organic pollutants (POPs) are recognized aspollutantsof global concern, but so far, information on the trends of legacyPOPs in the waters of the world has been missing due to logistical,analytical, and financial reasons. Passive samplers have emerged asan attractive alternative to active water sampling methods as theyaccumulate POPs, represent time-weighted average concentrations, andcan easily be shipped and deployed. As part of the AQUA-GAPS/MONET,passive samplers were deployed at 40 globally distributed sites between2016 and 2020, for a total of 21 freshwater and 40 marine deployments.Results from silicone passive samplers showed & alpha;-hexachlorocyclohexane(HCH) and & gamma;-HCH displaying the greatest concentrations in thenorthern latitudes/Arctic Ocean, in stark contrast to the more persistentpenta (PeCB)- and hexachlorobenzene (HCB), which approached equilibriumacross sampling sites. Geospatial patterns of polychlorinated biphenyl(PCB) aqueous concentrations closely matched original estimates ofproduction and use, implying limited global transport. Positive correlationsbetween log-transformed concentrations of & sigma;7PCB,& sigma;DDTs, & sigma;endosulfan, and & sigma;chlordane, but not & sigma;HCH,and the log of population density (p < 0.05) within5 and 10 km of the sampling sites also supported limited transportfrom used sites. These results help to understand the extent of globaldistribution, and eventually time-trends, of organic pollutants inaquatic systems, such as across freshwaters and oceans. Future deploymentswill aim to establish time-trends at selected sites while adding tothe geographical coverage.
ER  -

LOHMANN, Rainer, Branislav VRANA, Derek MUIR, Foppe SMEDES, Jaromír SOBOTKA, Eddy Y. ZENG, Lian-Jun BAO, Ian J. ALLAN, Peleg ASTRAHAN, Ricardo O. BARRA, Terry BIDLEMAN, Evgen DYKYI, Nicolas ESTOPPEY, Gilberto FILLMANN, Naomi GREENWOOD, Paul A. HELM, Liisa JANTUNEN, Sarit KASERZON, J. Vinicio MACIAS, Keith A. MARUYA, Francisco MOLINA, Brent NEWMAN, Raimon M. PRATS, Manolis TSAPAKIS, Mats TYSKLIND, Barend L. VAN DROOGE, Cameron J. VEAL a Charles S. WONG. Passive-Sampler-Derived PCB and OCP Concentrations in the Waters of the World─First Results from the AQUA-GAPS/MONET Network. \textit{Environmental Science and Technology}. American Chemical Society, 2023, roč.~57, č.~25, s.~9342-9352. ISSN~0013-936X. Dostupné z: https://dx.doi.org/10.1021/acs.est.3c01866.

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