a 2013

Study of Ge-As-Se chalcogenide glasses using laser desorption ionisation time-of-flight mass spectrometry

ŠVIHLOVÁ, Katarína; Lubomír PROKEŠ; Milan ALBERTI; Petr NĚMEC; Josef HAVEL et al.

Základní údaje

Originální název

Study of Ge-As-Se chalcogenide glasses using laser desorption ionisation time-of-flight mass spectrometry

Autoři

ŠVIHLOVÁ, Katarína; Lubomír PROKEŠ; Milan ALBERTI; Petr NĚMEC a Josef HAVEL

Vydání

2013

Další údaje

Jazyk

angličtina

Typ výsledku

Konferenční abstrakt

Obor

10406 Analytical chemistry

Stát vydavatele

Slovensko

Utajení

není předmětem státního či obchodního tajemství

Označené pro přenos do RIV

Ano

Kód RIV

RIV/00216224:14310/13:00069634

Organizační jednotka

Přírodovědecká fakulta

ISSN

Klíčová slova anglicky

chalcogenide glasses; Ge-As-Se; LDI ToF MS
Změněno: 6. 3. 2014 18:08, Mgr. Katarína Šútorová, Ph.D.

Anotace

V originále

Chalcogenide glasses are advanced materials with many applications in the field of infrared optics and electronics. The Ge-As-Se system belongs to group of glasses which are distinguished from other materials by large glass-forming region as well as tuning their photosensitivity/photostability. The glasses and amorphous thin films from Ge-As-Se system were already studied via several methods, however the plasma chemistry which is of high importance for thin films growth via plasma techniques is not understood yet. Therefore, in this work Ge-As-Se glasses were manufactured and their interaction with high energy laser pulses was studied using laser desorption ionisation time-of-flight mass spectrometry. It was shown in previous papers that clusters ablated from the solid glass posses to a certain extend part of the original structure and thus information about the structural patterns of solid glass can be obtained. The spectra are quite complex and often result of several clusters overlap. Because germanium always contains some hydrogen, GemAsnSeo clusters observed are overlayed with hydrogenated GemAsnSeoHx species. The stoichiometry was proposed analysing isotopic envelopes and via computer modeling with respect to composition of original chalcogenide glasses. Chalcogenide glasses are advanced materials with many applications in the field of infrared optics and electronics. The Ge-As-Se system belongs to group of glasses which are distinguished from other materials by large glass-forming region as well as tuning their photosensitivity/photostability. The glasses and amorphous thin films from Ge-As-Se system were already studied via several methods [1, 2], however the plasma chemistry which is of high importance for thin films growth via plasma techniques is not understood yet. Therefore, in this work Ge-As-Se glasses were manufactured and their interaction with high energy laser pulses was studied using laser desorption ionisation time-of-flight mass spectrometry. It was shown in previous papers [3, 4] that clusters ablated from the solid glass posses to a certain extend part of the original structure and thus information about the structural patterns of solid glass can be obtained. The spectra are quite complex and often result of several clusters overlap. Because germanium always contains some hydrogen, GemAsnSeo clusters observed are overlayed with hydrogenated GemAsnSeoHx species. The stoichiometry was proposed analysing isotopic envelopes and via computer modeling with respect to composition of original chalcogenide glasses.

Návaznosti

CZ.1.05/2.1.00/03.0086, interní kód MU
Název: CEPLANT - Regionální VaV centrum pro nízkonákladové plazmové a nanotechnologické povrchové úpravy
Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, CEPLANT - Regionální VaV centrum pro nízkonákladové plazmové a nanotechnologické povrchové úpravy, 2.1 Regionální VaV centra
ED2.1.00/03.0086, projekt VaV
Název: Regionální VaV centrum pro nízkonákladové plazmové a nanotechnologické povrchové úpravy
MSM0021622411, záměr
Název: Studium a aplikace plazmochemických reakcí v neizotermickém nízkoteplotním plazmatu a jeho interakcí s povrchem pevných látek
Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Studium a aplikace plazmochemických reakcí v neizotermickém nízkoteplotním plazmatu a jeho interakcí s povrchem pevných látek