Does an analysis of polychlorinated biphenyl (PCB) distribution
in mountain soils across China reveal a latitudinal
fractionation paradox?

J 2014

Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox?

ZHENG, Qian, Luca NIZZETTO, Marie Daniëlle MULDER, Ondřej SÁŇKA, Gerhard LAMMEL et. al.

Základní údaje

Originální název

Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox?

Autoři

ZHENG, Qian (156 Čína), Luca NIZZETTO (380 Itálie, garant, domácí), Marie Daniëlle MULDER (528 Nizozemské království, domácí), Ondřej SÁŇKA (203 Česká republika, domácí), Gerhard LAMMEL (276 Německo, domácí), Jun LI (156 Čína), Haijian BING (156 Čína), Xin LIU (156 Čína), Yishan JIANG (156 Čína), Chunlin LUO (156 Čína) a Gan ZHANG (156 Čína)

Vydání

Environmental Pollution, OXFORD, OXON, ENGLAND, ELSEVIER SCI LTD, 2014, 0269-7491

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Velká Británie a Severní Irsko

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 4.143

Kód RIV

RIV/00216224:14310/14:00079391

Organizační jednotka

Přírodovědecká fakulta

DOI

http://dx.doi.org/10.1016/j.envpol.2014.08.021

UT WoS

000344437600015

Klíčová slova anglicky

POP; PCB; Fractionation; Cold trapping; Mountain; Soil; Latitude; Forest

Štítky

AKR, rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 5. 3. 2015 12:43, Ing. Filip Vaculovič

Anotace

V originále

Organic and mineral soil horizons from forests in 30 mountains across China were analysed for polychlorinated biphenyl (PCB). Soil total organic carbon (TOC) content was a key determinant of PCB distribution explaining over 90% of the differences between organic and mineral soils, and between 30% and 60% of the variance along altitudinal and regional transects. The residual variance (after normalization by TOC) was small. Tri- to tetra-CB levels were higher in the South in relation to high source density and precipitation. Heavier congeners were instead more abundant at mid/high-latitudes where the advection pattern was mainly from long range transport. This resulted in a latitudinal fractionation opposite to theoretical expectations. The study showed that exposure to sources with different characteristics, and possibly accumulation/degradation trends of different congeners in soils being out-of-phase at different latitudes, can lead to an unsteady large scale distribution scenario conflicting with the thermodynamic equilibrium perception. (C) 2014 Elsevier Ltd. All rights reserved.

Návaznosti

LM2011028, projekt VaV

Název: RECETOX ? Národní infrastruktura pro výzkum toxických látek v prostředí

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, RECETOX Národní infrastruktura pro výzkum toxických látek v prostředí

Citovat

ZHENG, Qian, Luca NIZZETTO, Marie Daniëlle MULDER, Ondřej SÁŇKA, Gerhard LAMMEL, Jun LI, Haijian BING, Xin LIU, Yishan JIANG, Chunlin LUO a Gan ZHANG. Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox? Environmental Pollution. OXFORD, OXON, ENGLAND: ELSEVIER SCI LTD, 2014, roč. 195, DEC 2014, s. 115-122. ISSN 0269-7491. Dostupné z: https://dx.doi.org/10.1016/j.envpol.2014.08.021.

@article{1229196,
   author = {Zheng, Qian and Nizzetto, Luca and Mulder, Marie Daniëlle and Sáňka, Ondřej and Lammel, Gerhard and Li, Jun and Bing, Haijian and Liu, Xin and Jiang, Yishan and Luo, Chunlin and Zhang, Gan},
   article_location = {OXFORD, OXON, ENGLAND},
   article_number = {DEC 2014},
   doi = {http://dx.doi.org/10.1016/j.envpol.2014.08.021},
   keywords = {POP; PCB; Fractionation; Cold trapping; Mountain; Soil; Latitude; Forest},
   language = {eng},
   issn = {0269-7491},
   journal = {Environmental Pollution},
   title = {Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox?},
   url = {http://www.sciencedirect.com/science/article/pii/S0269749114003601},
   volume = {195},
   year = {2014}
}

TY  - JOUR
ID  - 1229196
AU  - Zheng, Qian - Nizzetto, Luca - Mulder, Marie Daniëlle - Sáňka, Ondřej - Lammel, Gerhard - Li, Jun - Bing, Haijian - Liu, Xin - Jiang, Yishan - Luo, Chunlin - Zhang, Gan
PY  - 2014
TI  - Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox?
JF  - Environmental Pollution
VL  - 195
IS  - DEC 2014
SP  - 115-122
EP  - 115-122
PB  - ELSEVIER SCI LTD
SN  - 02697491
KW  - POP
KW  - PCB
KW  - Fractionation
KW  - Cold trapping
KW  - Mountain
KW  - Soil
KW  - Latitude
KW  - Forest
UR  - http://www.sciencedirect.com/science/article/pii/S0269749114003601
L2  - http://www.sciencedirect.com/science/article/pii/S0269749114003601
N2  - Organic and mineral soil horizons from forests in 30 mountains across China were analysed for polychlorinated biphenyl (PCB). Soil total organic carbon (TOC) content was a key determinant of PCB distribution explaining over 90% of the differences between organic and mineral soils, and between 30% and 60% of the variance along altitudinal and regional transects. The residual variance (after normalization by TOC) was small. Tri- to tetra-CB levels were higher in the South in relation to high source density and precipitation. Heavier congeners were instead more abundant at mid/high-latitudes where the advection pattern was mainly from long range transport. This resulted in a latitudinal fractionation opposite to theoretical expectations. The study showed that exposure to sources with different characteristics, and possibly accumulation/degradation trends of different congeners in soils being out-of-phase at different latitudes, can lead to an unsteady large scale distribution scenario conflicting with the thermodynamic equilibrium perception. (C) 2014 Elsevier Ltd. All rights reserved.
ER  -

ZHENG, Qian, Luca NIZZETTO, Marie Dani$\backslash$''elle MULDER, Ondřej SÁŇKA, Gerhard LAMMEL, Jun LI, Haijian BING, Xin LIU, Yishan JIANG, Chunlin LUO a Gan ZHANG. Does an analysis of polychlorinated biphenyl (PCB) distribution in mountain soils across China reveal a latitudinal fractionation paradox? \textit{Environmental Pollution}. OXFORD, OXON, ENGLAND: ELSEVIER SCI LTD, 2014, roč.~195, DEC 2014, s.~115-122. ISSN~0269-7491. Dostupné z: https://dx.doi.org/10.1016/j.envpol.2014.08.021.

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