Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized,
Abundant, Ubiquitous Pollutant in the Built and Natural
Environment

J 2018

Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment

VENIER, Marta; William A. STUBBINGS; Jiehong GUO; Kevin ROMANAK; Linh V. NGUYEN et al.

Základní údaje

Originální název

Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment

Autoři

VENIER, Marta; William A. STUBBINGS; Jiehong GUO; Kevin ROMANAK; Linh V. NGUYEN; Liisa M. JANTUNEN; Lisa Emily MELYMUK ; Victoria ARRANDALE; Miriam L. DIAMOND a Ronald A. HITES

Vydání

ENVIRONMENTAL SCIENCE & TECHNOLOGY, WASHINGTON, AMER CHEMICAL SOC, 2018, 0013-936X

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Spojené státy

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 7.149

Označené pro přenos do RIV

Ano

Kód RIV

RIV/00216224:14310/18:00106142

Organizační jednotka

Přírodovědecká fakulta

Klíčová slova anglicky

RESOLUTION MASS-SPECTROMETRY; BROMINATED FLAME RETARDANTS; HOUSE-DUST; WASTE; IDENTIFICATION; MIGRATION; PRODUCTS

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 10. 2. 2019 21:02, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

Using high-resolution mass spectrometry, we identified tri(2,4-di-t-butylphenyl) phosphate (TDTBPP) in e-waste dust. This is a previously unsuspected pollutant that had not been reported before in the environment. To assess its abundance in the environment, we measured its concentration in e-waste dust, house dust, sediment from the Chicago Ship and Sanitary Canal, Indiana Harbor water filters, and filters from high-volume air samplers deployed in Chicago, IL. To provide a context for interpreting these quantitative results, we also measured the concentrations of triphenyl phosphate (TPhP), a structurally similar compound, in these samples. Median concentrations of TDTBPP and TPhP were 14 400 and 41 500 ng/g, respectively, in e-waste dust and 4900 and 2100 ng/g, respectively, in house dust. TDTBPP was detected in sediment, water, and air with median concentrations of 527 ng/g, 3700 pg/L, and 149 pg/m(3), respectively. TDTBPP concentrations were generally higher or comparable to those of TPhP in all media analyzed, except for the e-waste dust. Exposure from dust ingestion and dermal absorption in the e-waste recycling facility and in homes was calculated. TDTBPP exposure was 571 ng/kg bw/day in the e-waste recycling facility (pro-rated for an 8-h shift), and 536 ng/kg bw and 7550 ng/kg bw/day for adults and toddlers, respectively, in residential environments.

Návaznosti

LH12074, projekt VaV

Název: Nové typy bromovaných zpomalovačů hoření v prostředí (Akronym: BFR-ENVI)

Investor: Ministerstvo školství, mládeže a tělovýchovy ČR, Nové typy bromovaných zpomalovačů hoření v prostředí

Citovat

VENIER, Marta; William A. STUBBINGS; Jiehong GUO; Kevin ROMANAK; Linh V. NGUYEN; Liisa M. JANTUNEN; Lisa Emily MELYMUK; Victoria ARRANDALE; Miriam L. DIAMOND a Ronald A. HITES. Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment. ENVIRONMENTAL SCIENCE & TECHNOLOGY. WASHINGTON: AMER CHEMICAL SOC, 2018, roč. 52, č. 22, s. 12997-13003. ISSN 0013-936X. Dostupné z: https://doi.org/10.1021/acs.est.8b02939.

@article{1495618,
   author = {Venier, Marta and Stubbings, William A. and Guo, Jiehong and Romanak, Kevin and Nguyen, Linh V. and Jantunen, Liisa M. and Melymuk, Lisa Emily and Arrandale, Victoria and Diamond, Miriam L. and Hites, Ronald A.},
   article_location = {WASHINGTON},
   article_number = {22},
   doi = {https://doi.org/10.1021/acs.est.8b02939},
   keywords = {RESOLUTION MASS-SPECTROMETRY; BROMINATED FLAME RETARDANTS; HOUSE-DUST; WASTE; IDENTIFICATION; MIGRATION; PRODUCTS},
   language = {eng},
   issn = {0013-936X},
   journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY},
   title = {Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment},
   url = {https://pubs.acs.org/doi/10.1021/acs.est.8b02939},
   volume = {52},
   year = {2018}
}

TY  - JOUR
ID  - 1495618
AU  - Venier, Marta - Stubbings, William A. - Guo, Jiehong - Romanak, Kevin - Nguyen, Linh V. - Jantunen, Liisa M. - Melymuk, Lisa Emily - Arrandale, Victoria - Diamond, Miriam L. - Hites, Ronald A.
PY  - 2018
TI  - Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment
JF  - ENVIRONMENTAL SCIENCE & TECHNOLOGY
VL  - 52
IS  - 22
SP  - 12997-13003
EP  - 12997-13003
PB  - AMER CHEMICAL SOC
SN  - 0013936X
KW  - RESOLUTION MASS-SPECTROMETRY
KW  - BROMINATED FLAME RETARDANTS
KW  - HOUSE-DUST
KW  - WASTE
KW  - IDENTIFICATION
KW  - MIGRATION
KW  - PRODUCTS
UR  - https://pubs.acs.org/doi/10.1021/acs.est.8b02939
L2  - https://pubs.acs.org/doi/10.1021/acs.est.8b02939
N2  - Using high-resolution mass spectrometry, we identified tri(2,4-di-t-butylphenyl) phosphate (TDTBPP) in e-waste dust. This is a previously unsuspected pollutant that had not been reported before in the environment. To assess its abundance in the environment, we measured its concentration in e-waste dust, house dust, sediment from the Chicago Ship and Sanitary Canal, Indiana Harbor water filters, and filters from high-volume air samplers deployed in Chicago, IL. To provide a context for interpreting these quantitative results, we also measured the concentrations of triphenyl phosphate (TPhP), a structurally similar compound, in these samples. Median concentrations of TDTBPP and TPhP were 14 400 and 41 500 ng/g, respectively, in e-waste dust and 4900 and 2100 ng/g, respectively, in house dust. TDTBPP was detected in sediment, water, and air with median concentrations of 527 ng/g, 3700 pg/L, and 149 pg/m(3), respectively. TDTBPP concentrations were generally higher or comparable to those of TPhP in all media analyzed, except for the e-waste dust. Exposure from dust ingestion and dermal absorption in the e-waste recycling facility and in homes was calculated. TDTBPP exposure was 571 ng/kg bw/day in the e-waste recycling facility (pro-rated for an 8-h shift), and 536 ng/kg bw and 7550 ng/kg bw/day for adults and toddlers, respectively, in residential environments.
ER  -

VENIER, Marta; William A. STUBBINGS; Jiehong GUO; Kevin ROMANAK; Linh V. NGUYEN; Liisa M. JANTUNEN; Lisa Emily MELYMUK; Victoria ARRANDALE; Miriam L. DIAMOND a Ronald A. HITES. Tri(2,4-di-t-butylphenyl) Phosphate: A Previously Unrecognized, Abundant, Ubiquitous Pollutant in the Built and Natural Environment. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON: AMER CHEMICAL SOC, 2018, roč.~52, č.~22, s.~12997-13003. ISSN~0013-936X. Dostupné z: https://doi.org/10.1021/acs.est.8b02939.

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