A Simple Teabag Equilibrium Passive Sampler using hydrophilic
divinylbenzene sorbent for contaminants of emerging concern in
the marine environment

J 2021

A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment

VANRYCKEGHEM, Francis; Steve HUYSMAN; Foppe SMEDES; Herman VAN LANGENHOVE; Lynn VANHAECKE et. al.

Základní údaje

Originální název

A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment

Autoři

VANRYCKEGHEM, Francis (56 Belgie); Steve HUYSMAN (56 Belgie); Foppe SMEDES (528 Nizozemské království, garant, domácí); Herman VAN LANGENHOVE (56 Belgie); Lynn VANHAECKE (56 Belgie) a Kristof DEMEESTERE (56 Belgie)

Vydání

Science of the Total Environment, Amsterdam, Elsevier Science, 2021, 0048-9697

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Nizozemské království

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 10.754

Kód RIV

RIV/00216224:14310/21:00122209

Organizační jednotka

Přírodovědecká fakulta

DOI

https://doi.org/10.1016/j.scitotenv.2021.146055

UT WoS

000655615100019

EID Scopus

2-s2.0-85102123447

Klíčová slova anglicky

Micropollutant; Passive sampling; Sampling rate; Equilibrium partitioning; Teabag; Marine environment

Štítky

rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 6. 6. 2025 09:46, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

A promising concept for sampling contaminants of emerging concern (CECs) using a home-made Simple Teabag Equilibrium Passive Sampler (STEPS) containing hydrophilic divinylbenzene (h-DVB) sorbent is presented and evaluated for application in estuarine systems. The uptake of a multi-class mixture of CECs with a broad polarity range (Log P ranging from -0.1 to 9.9) was investigated in static exposure batch experiments. Sampling rates (R-s) and equilibrium partitioning coefficients (K-sw) were determined for up to 74 CECs. Fast uptake (R-s = 0.3-12 L d(-1)) was noticed and the STEPS attained equilibrium partitioning after 1 to 2 weeks of exposure, with Log K-sw ranging from 4.1 to 6.5 L kg(-1). Field application of this novel h-DVB containing STEPS, followed by ultra-high performance liquid chromatography coupled to high-resolution Orbitrap mass spectrometry, revealed the presence of up to 40 steroidal hormones, (alkyl)phenols, phthalates, pharmaceuticals, personal care products, and pesticides in the Belgian Part of the North Sea. The measured trace concentrations (from 0.003 ng L-1 to 1.9 mu g L-1) and good precision (average RSD < 30%, n = 3) demonstrate the STEPS as fit-for-purpose for micropollutant analysis in the marine environment.

Návaznosti

EF16_013/0001761, projekt VaV

Název: RECETOX RI

90051, velká výzkumná infrastruktura

Název: RECETOX II

Citovat

VANRYCKEGHEM, Francis; Steve HUYSMAN; Foppe SMEDES; Herman VAN LANGENHOVE; Lynn VANHAECKE a Kristof DEMEESTERE. A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment. Science of the Total Environment. Amsterdam: Elsevier Science, 2021, roč. 777, July 2021, s. 1-9. ISSN 0048-9697. Dostupné z: https://doi.org/10.1016/j.scitotenv.2021.146055.

@article{1789146,
   author = {Vanryckeghem, Francis and Huysman, Steve and Smedes, Foppe and Van Langenhove, Herman and Vanhaecke, Lynn and Demeestere, Kristof},
   article_location = {Amsterdam},
   article_number = {July 2021},
   doi = {https://doi.org/10.1016/j.scitotenv.2021.146055},
   keywords = {Micropollutant; Passive sampling; Sampling rate; Equilibrium partitioning; Teabag; Marine environment},
   language = {eng},
   issn = {0048-9697},
   journal = {Science of the Total Environment},
   title = {A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment},
   url = {https://www.sciencedirect.com/science/article/pii/S0048969721011220?via%3Dihub},
   volume = {777},
   year = {2021}
}

TY  - JOUR
ID  - 1789146
AU  - Vanryckeghem, Francis - Huysman, Steve - Smedes, Foppe - Van Langenhove, Herman - Vanhaecke, Lynn - Demeestere, Kristof
PY  - 2021
TI  - A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment
JF  - Science of the Total Environment
VL  - 777
IS  - July 2021
SP  - 1-9
EP  - 1-9
PB  - Elsevier Science
SN  - 00489697
KW  - Micropollutant
KW  - Passive sampling
KW  - Sampling rate
KW  - Equilibrium partitioning
KW  - Teabag
KW  - Marine environment
UR  - https://www.sciencedirect.com/science/article/pii/S0048969721011220?via%3Dihub
N2  - A promising concept for sampling contaminants of emerging concern (CECs) using a home-made Simple Teabag Equilibrium Passive Sampler (STEPS) containing hydrophilic divinylbenzene (h-DVB) sorbent is presented and evaluated for application in estuarine systems. The uptake of a multi-class mixture of CECs with a broad polarity range (Log P ranging from -0.1 to 9.9) was investigated in static exposure batch experiments. Sampling rates (R-s) and equilibrium partitioning coefficients (K-sw) were determined for up to 74 CECs. Fast uptake (R-s = 0.3-12 L d(-1)) was noticed and the STEPS attained equilibrium partitioning after 1 to 2 weeks of exposure, with Log K-sw ranging from 4.1 to 6.5 L kg(-1). Field application of this novel h-DVB containing STEPS, followed by ultra-high performance liquid chromatography coupled to high-resolution Orbitrap mass spectrometry, revealed the presence of up to 40 steroidal hormones, (alkyl)phenols, phthalates, pharmaceuticals, personal care products, and pesticides in the Belgian Part of the North Sea. The measured trace concentrations (from 0.003 ng L-1 to 1.9 mu g L-1) and good precision (average RSD < 30%, n = 3) demonstrate the STEPS as fit-for-purpose for micropollutant analysis in the marine environment.
ER  -

VANRYCKEGHEM, Francis; Steve HUYSMAN; Foppe SMEDES; Herman VAN LANGENHOVE; Lynn VANHAECKE a Kristof DEMEESTERE. A Simple Teabag Equilibrium Passive Sampler using hydrophilic divinylbenzene sorbent for contaminants of emerging concern in the marine environment. \textit{Science of the Total Environment}. Amsterdam: Elsevier Science, 2021, roč.~777, July 2021, s.~1-9. ISSN~0048-9697. Dostupné z: https://doi.org/10.1016/j.scitotenv.2021.146055.

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