Wide-scope target screening characterization of legacy and
emerging contaminants in the Danube River Basin by liquid and
gas chromatography coupled with high-resolution mass
spectrometry

J 2023

Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry

NG, Kelsey Kwong Pui; Nikiforos ALYGIZAKIS; Maria-Christina NIKA; Aikaterini GALANI; Peter OSWALD et al.

Základní údaje

Originální název

Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry

Autoři

Vydání

Water Research, OXFORD, PERGAMON-ELSEVIER SCIENCE LTD, 2023, 0043-1354

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Velká Británie a Severní Irsko

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 11.500

Označené pro přenos do RIV

Ano

Kód RIV

RIV/00216224:14310/23:00130848

Organizační jednotka

Přírodovědecká fakulta

Klíčová slova anglicky

Organic pollutants; Danube River Basin; Wastewater treatment plants; Target screening; Environmental risk assessment

Štítky

143180, rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 25. 5. 2023 20:28, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

A state-of-the-art wide-scope target screening of 2,362 chemicals and their transformation products (TPs) was performed in samples collected within the Joint Danube Survey 4 (JDS4) performed in 2019. The analysed contaminants of emerging concern (CECs) included three major categories: plant protection products (PPPs), industrial chemicals and pharmaceuticals and personal care products (PPCPs). In total, 586 CECs were detected in the samples including 158 PPPs, 71 industrial chemicals, 348 PPCPs, and 9 other chemicals. A wide-variety of sample matrices were collected including influent and effluent wastewater, groundwater, river water, sediment and biota. Forty-five CECs (19 PPPs, 8 industrial chemicals, 18 PPCPs) were detected at levels above their ecotoxicological thresholds (lowest predicted no-effect concentration (PNEC) values) in one or more of the investigated environmental compartments, indicating potential adverse effects on the impacted ecosystems. Among them 12 are legacy substances; 33 are emerging and qualify as potential Danube River Basin Specific Pollutants (RBSPs). Moreover, the efficiency of the wastewater treatment plants (WWTPs) was evaluated using 20 selected performance indicator chemicals. WWTPs showed effective removal (removal rate >= 80%) and me-dium removal (removal rate 25-80%) for 6 and 8 of the indicator chemicals, respectively. However, numerous contaminants passed the WWTPs with a lower removal rate. Further investigation on performance of WWTPs is suggested at catchment level to improve their removal efficiency. WWTP effluents are proven to be one of the major sources of contaminants in the Danube River Basin (DRB). Other sources include sewage discharges, in-dustrial and agricultural activities. Continuous monitoring of the detected CECs is suggested to ensure water quality of the studied area.

Návaznosti

859891, interní kód MU

Název: Best chemical risk assessment professionals for maximum Ecosystem Services benefit (Akronym: PRORISK)

Investor: Evropská unie, Best chemical risk assessment professionals for maximum Ecosystem Services benefit, MSCA Marie Skłodowska-Curie Actions (Excellent Science)

Citovat

NG, Kelsey Kwong Pui; Nikiforos ALYGIZAKIS; Maria-Christina NIKA; Aikaterini GALANI; Peter OSWALD; Martina OSWALDOVA; Lubos CIRKA; Uwe KUNKEL; Andre MACHERIUS; Manfred SENGL; Giulio MARIANI; Simona TAVAZZI; Helle SKEJO; Bernd M. GAWLIK; Nikolaos S. THOMAIDIS a Jaroslav SLOBODNÍK. Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry. Water Research. OXFORD: PERGAMON-ELSEVIER SCIENCE LTD, 2023, roč. 230, February 2023, s. 1-10. ISSN 0043-1354. Dostupné z: https://doi.org/10.1016/j.watres.2022.119539.

@article{2285699,
   author = {Ng, Kelsey Kwong Pui and Alygizakis, Nikiforos and Nika, MariaandChristina and Galani, Aikaterini and Oswald, Peter and Oswaldova, Martina and Cirka, Lubos and Kunkel, Uwe and Macherius, Andre and Sengl, Manfred and Mariani, Giulio and Tavazzi, Simona and Skejo, Helle and Gawlik, Bernd M. and Thomaidis, Nikolaos S. and Slobodník, Jaroslav},
   article_location = {OXFORD},
   article_number = {February 2023},
   doi = {https://doi.org/10.1016/j.watres.2022.119539},
   keywords = {Organic pollutants; Danube River Basin; Wastewater treatment plants; Target screening; Environmental risk assessment},
   language = {eng},
   issn = {0043-1354},
   journal = {Water Research},
   title = {Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry},
   url = {https://www.sciencedirect.com/science/article/pii/S0043135422014841?via%3Dihub},
   volume = {230},
   year = {2023}
}

TY  - JOUR
ID  - 2285699
AU  - Ng, Kelsey Kwong Pui - Alygizakis, Nikiforos - Nika, Maria-Christina - Galani, Aikaterini - Oswald, Peter - Oswaldova, Martina - Cirka, Lubos - Kunkel, Uwe - Macherius, Andre - Sengl, Manfred - Mariani, Giulio - Tavazzi, Simona - Skejo, Helle - Gawlik, Bernd M. - Thomaidis, Nikolaos S. - Slobodník, Jaroslav
PY  - 2023
TI  - Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry
JF  - Water Research
VL  - 230
IS  - February 2023
SP  - 1-10
EP  - 1-10
PB  - PERGAMON-ELSEVIER SCIENCE LTD
SN  - 00431354
KW  - Organic pollutants
KW  - Danube River Basin
KW  - Wastewater treatment plants
KW  - Target screening
KW  - Environmental risk assessment
UR  - https://www.sciencedirect.com/science/article/pii/S0043135422014841?via%3Dihub
N2  - A state-of-the-art wide-scope target screening of 2,362 chemicals and their transformation products (TPs) was performed in samples collected within the Joint Danube Survey 4 (JDS4) performed in 2019. The analysed contaminants of emerging concern (CECs) included three major categories: plant protection products (PPPs), industrial chemicals and pharmaceuticals and personal care products (PPCPs). In total, 586 CECs were detected in the samples including 158 PPPs, 71 industrial chemicals, 348 PPCPs, and 9 other chemicals. A wide-variety of sample matrices were collected including influent and effluent wastewater, groundwater, river water, sediment and biota. Forty-five CECs (19 PPPs, 8 industrial chemicals, 18 PPCPs) were detected at levels above their ecotoxicological thresholds (lowest predicted no-effect concentration (PNEC) values) in one or more of the investigated environmental compartments, indicating potential adverse effects on the impacted ecosystems. Among them 12 are legacy substances; 33 are emerging and qualify as potential Danube River Basin Specific Pollutants (RBSPs). Moreover, the efficiency of the wastewater treatment plants (WWTPs) was evaluated using 20 selected performance indicator chemicals. WWTPs showed effective removal (removal rate >= 80%) and me-dium removal (removal rate 25-80%) for 6 and 8 of the indicator chemicals, respectively. However, numerous contaminants passed the WWTPs with a lower removal rate. Further investigation on performance of WWTPs is suggested at catchment level to improve their removal efficiency. WWTP effluents are proven to be one of the major sources of contaminants in the Danube River Basin (DRB). Other sources include sewage discharges, in-dustrial and agricultural activities. Continuous monitoring of the detected CECs is suggested to ensure water quality of the studied area.
ER  -

NG, Kelsey Kwong Pui; Nikiforos ALYGIZAKIS; Maria-Christina NIKA; Aikaterini GALANI; Peter OSWALD; Martina OSWALDOVA; Lubos CIRKA; Uwe KUNKEL; Andre MACHERIUS; Manfred SENGL; Giulio MARIANI; Simona TAVAZZI; Helle SKEJO; Bernd M. GAWLIK; Nikolaos S. THOMAIDIS a Jaroslav SLOBODNÍK. Wide-scope target screening characterization of legacy and emerging contaminants in the Danube River Basin by liquid and gas chromatography coupled with high-resolution mass spectrometry. \textit{Water Research}. OXFORD: PERGAMON-ELSEVIER SCIENCE LTD, 2023, roč.~230, February 2023, s.~1-10. ISSN~0043-1354. Dostupné z: https://doi.org/10.1016/j.watres.2022.119539.

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