Spatial and Temporal Trends of Dissolved Polybrominated
Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic
Environment across Countries

J 2025

Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries

BAO, Lian-Jun; Branislav VRANA; Rainer LOHMANN; Jaromír SOBOTKA; Foppe SMEDES et al.

Základní údaje

Originální název

Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries

Autoři

Vydání

ENVIRONMENTAL SCIENCE & TECHNOLOGY, WASHINGTON, DC (USA), AMER CHEMICAL SOC, 2025, 0013-936X

Další údaje

Jazyk

angličtina

Typ výsledku

Článek v odborném periodiku

Obor

10511 Environmental sciences

Stát vydavatele

Spojené státy

Utajení

není předmětem státního či obchodního tajemství

Odkazy

URL

Impakt faktor

Impact factor: 11.300 v roce 2024

Označené pro přenos do RIV

Ano

Kód RIV

RIV/00216224:14310/25:00142672

Organizační jednotka

Přírodovědecká fakulta

Klíčová slova anglicky

AQUA-GAPS/MONET; passive sampling; halogenatedflame retardants; seawater and freshwater; anthropogenicactivity

Štítky

143180, rivok

Příznaky

Mezinárodní význam, Recenzováno

Změněno: 15. 2. 2026 09:27, Mgr. Michaela Hylsová, Ph.D.

Anotace

V originále

Measuring dissolved concentrations of polybrominated diphenyl ethers (PBDEs) and non-BDE flame retardants on a global scale provides critical insights into the effectiveness of the Stockholm Convention. In the present study, we deployed passive sampling devices at 43 seawater and freshwater sites covering 21 countries from 2016 to 2020. The detection frequencies were 20-94% for BDE congeners and 33-42% for dechlorane plus, higher than those (0-20%) for other target compounds. The median concentrations of dissolved Sigma 9PBDE (sum of BDE-28, -47, -66, -85, -99, -100, -153, -154, and -183) were 0.28 and 0.64 pg L-1 in seawater and freshwater, respectively. The concentrations of dissolved Sigma 9PBDE, along with published data, slightly increased before 2016 and remained steady from 2016 to 2018, indicating delayed effects of the global phaseout of technical Penta- and Octa-BDEs. The log-transformed concentrations of individual BDE congeners were better correlated with regional gross domestic product than with population density. The potential ecological risk of BDE-47 was low, and there was a lack of key risk indicators for other compounds. The present study documented the delayed response of the aquatic environment to the regulatory actions on reducing PBDE emissions.

Návaznosti

GX20-04676X, projekt VaV

Název: Holistická charakterizace expozice a potenciálních účinků komplexních směsí chemických látek ve vodním prostředí

Investor: Grantová agentura ČR, Holistická charakterizace expozice a potenciálních účinků komplexních směsí chemických látek ve vodním prostředí

857560, interní kód MU
(Kód CEP: EF17_043/0009632)

Název: CETOCOEN Excellence (Akronym: CETOCOEN Excellence)

Investor: Evropská unie, CETOCOEN Excellence, Spreading excellence and widening participation

90269, velká výzkumná infrastruktura

Název: RECETOX RI II

Citovat

BAO, Lian-Jun; Branislav VRANA; Rainer LOHMANN; Jaromír SOBOTKA; Foppe SMEDES; Derek MUIR; Ian J. ALLAN; Peleg ASTRAHAN; Terry BIDLEMAN; Denis CROWLEY; Evgen DYKYI; Nicolas ESTOPPEY; Gilberto FILLMANN; Liisa JANTUNEN; Sarit KASERZON; Keith A. MARUYA; Brendan MCHUGH; Brent NEWMAN; Raimon M. PRATS; Manolis TSAPAKIS; Rebecca SUTTON; Mats TYSKLIND; Barend L. VAN DROOGE; Charles S. WONG a Eddy Y. ZENG. Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries. ENVIRONMENTAL SCIENCE & TECHNOLOGY. WASHINGTON, DC (USA): AMER CHEMICAL SOC, 2025, roč. 59, č. 45, s. 24576-24586. ISSN 0013-936X. Dostupné z: https://doi.org/10.1021/acs.est.5c11506.

@article{2535249,
   author = {Bao, LianandJun and Vrana, Branislav and Lohmann, Rainer and Sobotka, Jaromír and Smedes, Foppe and Muir, Derek and Allan, Ian J. and Astrahan, Peleg and Bidleman, Terry and Crowley, Denis and Dykyi, Evgen and Estoppey, Nicolas and Fillmann, Gilberto and Jantunen, Liisa and Kaserzon, Sarit and Maruya, Keith A. and Mchugh, Brendan and Newman, Brent and Prats, Raimon M. and Tsapakis, Manolis and Sutton, Rebecca and Tysklind, Mats and Van Drooge, Barend L. and Wong, Charles S. and Zeng, Eddy Y.},
   article_location = {WASHINGTON, DC (USA)},
   article_number = {45},
   doi = {https://doi.org/10.1021/acs.est.5c11506},
   keywords = {AQUA-GAPS/MONET; passive sampling; halogenatedflame retardants; seawater and freshwater; anthropogenicactivity},
   language = {eng},
   issn = {0013-936X},
   journal = {ENVIRONMENTAL SCIENCE & TECHNOLOGY},
   title = {Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries},
   url = {https://pubs.acs.org/doi/10.1021/acs.est.5c11506},
   volume = {59},
   year = {2025}
}

TY  - JOUR
ID  - 2535249
AU  - Bao, Lian-Jun - Vrana, Branislav - Lohmann, Rainer - Sobotka, Jaromír - Smedes, Foppe - Muir, Derek - Allan, Ian J. - Astrahan, Peleg - Bidleman, Terry - Crowley, Denis - Dykyi, Evgen - Estoppey, Nicolas - Fillmann, Gilberto - Jantunen, Liisa - Kaserzon, Sarit - Maruya, Keith A. - Mchugh, Brendan - Newman, Brent - Prats, Raimon M. - Tsapakis, Manolis - Sutton, Rebecca - Tysklind, Mats - Van Drooge, Barend L. - Wong, Charles S. - Zeng, Eddy Y.
PY  - 2025
TI  - Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries
JF  - ENVIRONMENTAL SCIENCE & TECHNOLOGY
VL  - 59
IS  - 45
SP  - 24576-24586
EP  - 24576-24586
PB  - AMER CHEMICAL SOC
SN  - 0013936X
KW  - AQUA-GAPS/MONET
KW  - passive sampling
KW  - halogenatedflame retardants
KW  - seawater and freshwater
KW  - anthropogenicactivity
UR  - https://pubs.acs.org/doi/10.1021/acs.est.5c11506
N2  - Measuring dissolved concentrations of polybrominated diphenyl ethers (PBDEs) and non-BDE flame retardants on a global scale provides critical insights into the effectiveness of the Stockholm Convention. In the present study, we deployed passive sampling devices at 43 seawater and freshwater sites covering 21 countries from 2016 to 2020. The detection frequencies were 20-94% for BDE congeners and 33-42% for dechlorane plus, higher than those (0-20%) for other target compounds. The median concentrations of dissolved Sigma 9PBDE (sum of BDE-28, -47, -66, -85, -99, -100, -153, -154, and -183) were 0.28 and 0.64 pg L-1 in seawater and freshwater, respectively. The concentrations of dissolved Sigma 9PBDE, along with published data, slightly increased before 2016 and remained steady from 2016 to 2018, indicating delayed effects of the global phaseout of technical Penta- and Octa-BDEs. The log-transformed concentrations of individual BDE congeners were better correlated with regional gross domestic product than with population density. The potential ecological risk of BDE-47 was low, and there was a lack of key risk indicators for other compounds. The present study documented the delayed response of the aquatic environment to the regulatory actions on reducing PBDE emissions.
ER  -

BAO, Lian-Jun; Branislav VRANA; Rainer LOHMANN; Jaromír SOBOTKA; Foppe SMEDES; Derek MUIR; Ian J. ALLAN; Peleg ASTRAHAN; Terry BIDLEMAN; Denis CROWLEY; Evgen DYKYI; Nicolas ESTOPPEY; Gilberto FILLMANN; Liisa JANTUNEN; Sarit KASERZON; Keith A. MARUYA; Brendan MCHUGH; Brent NEWMAN; Raimon M. PRATS; Manolis TSAPAKIS; Rebecca SUTTON; Mats TYSKLIND; Barend L. VAN DROOGE; Charles S. WONG a Eddy Y. ZENG. Spatial and Temporal Trends of Dissolved Polybrominated Diphenyl Ethers and Non-BDE Flame Retardants in the Aquatic Environment across Countries. \textit{ENVIRONMENTAL SCIENCE \&{}amp; TECHNOLOGY}. WASHINGTON, DC (USA): AMER CHEMICAL SOC, 2025, roč.~59, č.~45, s.~24576-24586. ISSN~0013-936X. Dostupné z: https://doi.org/10.1021/acs.est.5c11506.

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